$Rev:: 532 $ $Date:: 2011-12-05#$ 1 0 0 0 9.223700+4 2.350124+2 1 1 0 39234 1451 1 0.000000+0 1.000000+0 0 0 0 69234 1451 2 1.000000+0 3.000000+7 1 0 10 79234 1451 3 0.000000+0 0.000000+0 0 0 476 869234 1451 4 92-U -237 LANL EVAL-FEB09 P.G.Young, M.B.Chadwick 9234 1451 5 DIST- REV1- 20111222 9234 1451 6 ----ENDF/B-VII.1 MATERIAL 9234 REVISION 1 9234 1451 7 -----INCIDENT NEUTRON DATA 9234 1451 8 ------ENDF-6 FORMAT 9234 1451 9 9234 1451 10 AUG11 Added MT458 fission energy release data based on R. Vogt 9234 1451 11 Energy-Dependent Fission Q Values Generalized for All Actinides 9234 1451 12 Oct 8, 2008 report LLNL-TR-407620 9234 1451 13 9234 1451 14 **************************************************************** 9234 1451 15 12/09/2010 S.T. Holloway on behalf of LANL 9234 1451 16 Reverted MF=1/5, MT=455 Delayed-neutron 6-grp data to 9234 1451 17 ENDF/B-VI.8 values. 9234 1451 18 **************************************************************** 9234 1451 19 9234 1451 20 MOD 3C - ADOPT JENDL-3.3 RESONANCE PARAMETERS AND MINOR 9234 1451 21 ADJUSTMENT OF (N,F) CROSS SECTION BELOW 4 MeV. 9234 1451 22 [3-06-2009] 9234 1451 23 9234 1451 24 1. We replaced the resolved and unresolved resonance parameters 9234 1451 25 with the parameters from the JENDL-3.3 evaluation/1/. We 9234 1451 26 modified the unresolved resonace parameters slightly to maintain 9234 1451 27 the ENDF/B-VII.0 unresolved energy cutoff of 0.01 MeV and to join 9234 1451 28 with the smooth cross sections above 0.01 MeV. 9234 1451 29 9234 1451 30 2. We adjusted the (n,f) cross section between 0.01 and 4 MeV to 9234 1451 31 give a higher cross section in the 1-2 MeV range, consistent with 9234 1451 32 systematics by Behrens/2/, and to smoothly join with the cross 9234 1451 33 section at the unresolved resonance region cutoff. 9234 1451 34 9234 1451 35 REFERENCES 9234 1451 36 /1/ T. Nakagawa, JENDL-3.3 evaluation (2002). 9234 1451 37 /2/ J. Behrens, NSE,63,250,1977 9234 1451 38 9234 1451 39 **************************************************************** 9234 1451 40 9234 1451 41 MOD 3B - NEW GNASH ANALYSIS REVISED FOR SURROGATE (n,f) DATA 9234 1451 42 [2-25-2006] 9234 1451 43 9234 1451 44 1. We revised our GNASH analysis (describe below under MOD 3) 9234 1451 45 to better represent the surrogate (n,f) fission cross section 9234 1451 46 data of W.Younes and H.C. Britt (UCRL-TR-212600, May 31, 2005) 9234 1451 47 and J.T.Burke et al. (UCRL-TR-214631, August 16, 2005). The only 9234 1451 48 changes to parameters were to the fission barrier heights. Also a 9234 1451 49 newer version of mass tables was used (Reference Input Parameter 9234 1451 50 Library-2, RIPL-2, 2005) in the GNASH calculations. 9234 1451 51 9234 1451 52 2. The following MF=3 sections were replaced with the new 9234 1451 53 analysis: MT=4,16,17,18,37,91, and 102. The following MF=6 9234 1451 54 sections were replaced with the new analysis: MT=16,17,37, and 9234 1451 55 91. 9234 1451 56 9234 1451 57 3. The radiative capture width in the resolved and unresolved 9234 1451 58 resonance regions was changed from 34.56 meV to 23 meV, which 9234 1451 59 conforms to the value in the RIPL-2 data base. 9234 1451 60 9234 1451 61 **************************************************************** 9234 1451 62 9234 1451 63 MOD 3A - INCORPORATION OF REVISED DELAYED NEUTRON DATA 9234 1451 64 W. B. WILSON [2/28/05] 9234 1451 65 9234 1451 66 New DN 6-gp parameters from CINDER'90 summation calculations are 9234 1451 67 available. The CINDER calculations are based on a new CINDER 9234 1451 68 library in which beta-decay half-lives and beta-delayed neutron- 9234 1451 69 emission probablities are obtained from the evaluated experimental9234 1451 70 data file NuBase2003 (G. Audi, O. Bersillon, J. Blanchot, and 9234 1451 71 A. H. Wapstra, Nuclear Physics A729 (2003) p. 3-129), when avail- 9234 1451 72 able there. When experimental data are not available there they 9234 1451 73 are calculated in a model where allowed Gamow-Teller decays are 9234 1451 74 treated in a microscopic quasi-particle random-phase approximation9234 1451 75 (QRPA) and the first forbidden decays are treated in the statis- 9234 1451 76 tical gross theory (P. Moller, B. Pfeiffer, and K.-L. Kratz, Phys.9234 1451 77 Rev. C. 67 (2003) 055802). Further refinements are anticipated 9234 1451 78 before the final release of ENDF-7. 9234 1451 79 9234 1451 80 **************************************************************** 9234 1451 81 9234 1451 82 MOD 3 - PRELIMINARY EVALUATION OF n + 237U REACTIONS 9234 1451 83 9234 1451 84 P. G. Young and M. B. Chadwick 9234 1451 85 9234 1451 86 Theoretical Division 9234 1451 87 Los Alamos National Laboratory 9234 1451 88 Los Alamos, NM 87545 9234 1451 89 September, 2000 9234 1451 90 9234 1451 91 I. SUMMARY 9234 1451 92 9234 1451 93 The cross section data file for neutron reactions with 237U 9234 1451 94 has been reevaluated over the incident neutron energy range from 9234 1451 95 10-5 eV to 30 MeV. This work builds upon an earlier Los Alamos 9234 1451 96 evaluation (Yo94) that featured replacement of all cross section 9234 1451 97 data above 10 keV with results from a new theoretical analysis. 9234 1451 98 The present analysis updates the cross sections and continuum 9234 1451 99 energy-angle distributions with results from a systematic 9234 1451 100 analysis of 232,233,234,235,236,238U + n reactions. 9234 1451 101 9234 1451 102 Details of the present analysis are given in the sections 9234 1451 103 that follow. Some general features of the work are: 9234 1451 104 9234 1451 105 1. The ENDF/B-VI n + 237U resonance parameters were adopted at 9234 1451 106 neutron energies below 10 keV with modification of the fission 9234 1451 107 channel to better agree with data. The resonance analysis was 9234 1451 108 suitably joined with the present analysis at 10 keV. 9234 1451 109 9234 1451 110 2. A systematic analysis was performed of uranium isotopes 9234 1451 111 between 232U and 238U. An isospin-dependent coupled-channel 9234 1451 112 optical model potential was developed for the uranium isotopes 9234 1451 113 and was used to calculate the n + 237U neutron total cross 9234 1451 114 section, elastic and inelastic scattering cross sections, 9234 1451 115 elastic scattering angular distributions, and reaction cross 9234 1451 116 sections. Transmission coefficients were obtained from the 9234 1451 117 optical model for theoretical calculations with reaction theory 9234 1451 118 codes. 9234 1451 119 9234 1451 120 3. Prompt nubar and the fission neutron spectra were taken from 9234 1451 121 the existing ENDF/B-VI evaluation. 9234 1451 122 9234 1451 123 4. Angular distributions of (n,n') reactions were carried over 9234 1451 124 from the 1994 evaluation (Yo94). Those distributions were 9234 1451 125 obtained from a similar coupled-channels optical potential. 9234 1451 126 9234 1451 127 II. THEORETICAL ANALYSIS 9234 1451 128 9234 1451 129 The basic approach followed was to fit the available 9234 1451 130 experimental data for (n,f), (n,g), (n,xn), and other reactions 9234 1451 131 for the stable uranium isotopes using nuclear models, and to 9234 1451 132 then use reasonable extrapolations of the parameters to infer 9234 1451 133 cross sections for 237U. To perform the analysis, we utilized 9234 1451 134 the Hauser-Feshbach reaction theory code COMNUC, the Hauser- 9234 1451 135 Feshbach/preequilibrium reaction theory code GNASH, and the 9234 1451 136 coupled-channels optical model code ECIS. 9234 1451 137 9234 1451 138 A. Optical Model 9234 1451 139 9234 1451 140 The deformed optical model potential was obtained by 9234 1451 141 considering several coupled-channel parameterizations developed 9234 1451 142 from n + 235,238U and 239Pu experimental data , several of which 9234 1451 143 were used in ENDF/B-VI evaluations. The Harwell potential by 9234 1451 144 Madland and Young (Ma78), the Bruyeres-le-Chatel (BRC) potential 9234 1451 145 by Lagrange (Ha82), and a modified version of the BRC potential 9234 1451 146 by Arthur and Young (Yo88, Yo92a) were examined. Isospin 9234 1451 147 corrections were applied to all the potentials to adapt them for 9234 1451 148 the various U isotopes. Corrections from the measured to the 9234 1451 149 unmeasured cases were made in the deformation parameters b2 and 9234 1451 150 b4, using a simple model by D. Madland to calculate deformation 9234 1451 151 parameters for targets without experimental information from 9234 1451 152 deformations given in the extensive Nix-Moller mass analysis. 9234 1451 153 For the optical model potential, we chose to use an isospin 9234 1451 154 version of the BRC potential (Ha82), which was inferred from 9234 1451 155 Lagrange's results for individual nuclides. The lowest three 9234 1451 156 members of the 1/2+ ground state rotational band were included 9234 1451 157 in the calculations, that is, the 3/2+ and 5/2+ states at Ex = 9234 1451 158 11 and 56 keV were coupled with the 1/2+ ground state. All of 9234 1451 159 the potentials considered gave total and reaction cross sections 9234 1451 160 that were reasonably consistent, so the selection was based 9234 1451 161 mainly on the fact that the BRC potential gave better agreement 9234 1451 162 with fission cross sections for odd U isotopes (233,235U) at 9234 1451 163 lower energies. 9234 1451 164 9234 1451 165 B. Reaction Theory Calculations 9234 1451 166 9234 1451 167 The Hauser-Feshbach statistical calculations were performed 9234 1451 168 with the COMNUC (Du70) and GNASH (Yo92b) codes. Both codes 9234 1451 169 include a double-humped fission barrier model, using uncoupled 9234 1451 170 oscillators for the barrier representation in GNASH and coupled 9234 1451 171 or uncoupled oscillators in COMNUC, as described by Arthur 9234 1451 172 (Ar82a). The COMNUC calculations include the possibility of 9234 1451 173 width-fluctuation corrections and corrections for class II 9234 1451 174 fluctuations, which are needed at lower energies, whereas GNASH 9234 1451 175 provides the preequilibrium corrections that are required at 9234 1451 176 higher energies. Accordingly, COMNUC was used in the 9234 1451 177 calculations below about 0.5 MeV, utilizing a non-resonant model 9234 1451 178 and including class II fluctuations, and the GNASH code was 9234 1451 179 employed at higher energies using two uncoupled oscillators in 9234 1451 180 the fission calculations. 9234 1451 181 Each compound nucleus formed in the calculations is permitted 9234 1451 182 to decay through the fission channel, by neutron emission, and 9234 1451 183 by gamma-ray emission. Neutron transmission coefficients for 9234 1451 184 the Hauser-Feshbach calculations are obtained from the coupled- 9234 1451 185 channel optical model. Gamma ray transmission coefficients are 9234 1451 186 obtained from gamma-ray strength functions calculated with the 9234 1451 187 generalized Lorentzian model of Kopecky and Uhl (Ko90). 9234 1451 188 Transmission coefficients for fission are calculated from the 9234 1451 189 fission model summarized here and detailed in Yo92b. 9234 1451 190 Gilbert and Cameron (Gi70) phenomenological level density 9234 1451 191 functions were used to represent continuum levels at ground- 9234 1451 192 state deformations, appropriately matched to available 9234 1451 193 experimental structure data at lower excitation energies. 9234 1451 194 Multiplicative factors were applied to the level density 9234 1451 195 functions to account for enhancements in the fission transition 9234 1451 196 state densities at the fission barriers due to increased 9234 1451 197 asymmetry conditions, and the continuum level densities were 9234 1451 198 matched to the discrete fission transition states at each 9234 1451 199 barrier. The discrete fission transition state spectra were 9234 1451 200 calculated from bandhead information taken from calculations and 9234 1451 201 compilations by Britt (Br82). 9234 1451 202 Initial values of fission barrier parameters were taken from 9234 1451 203 the work of Britt (Br82,Ba74), and we used default level density 9234 1451 204 parameters of Gilbert and Cameron for all ground state nuclei. 9234 1451 205 We only modified the Britt-Back parameters in very simple ways 9234 1451 206 in order to facilitate extrapolation of the parameters. Our 9234 1451 207 modifications were limited to minor adjustments of the fission 9234 1451 208 barrier heights, the pairing energy at the fission barriers 9234 1451 209 (although we usually used the Gilbert-Cameron values), and the 9234 1451 210 level matching of the temperature region of the continuum level 9234 1451 211 densities at the fission saddles. The barrier parameters for 9234 1451 212 238U were checked by calculating the fission probability for the 9234 1451 213 236U(t,pf)238U reaction, as was done by Arthur in an earlier 9234 1451 214 analysis (Ar82b). Note that these calculations were performed 9234 1451 215 with COMNUC using a direct reaction (t,pf) spin distribution in 9234 1451 216 the analysis (Ar82c). 9234 1451 217 We fit the experimental (n,f) and (n,g) cross sections for 9234 1451 218 all stable isotopes over the energy region of first-chance 9234 1451 219 fission using the COMNUC model code. Experimental data exists 9234 1451 220 for targets of 232U, 233U, 234U, 235U, 236U, and 238U, which 9234 1451 221 allowed us to infer fission barrier parameters and gamma-ray 9234 1451 222 strength functions for the compound systems of 233U, 234U, 235U, 9234 1451 223 236U, 237U, and 239U. Using the parameters determined from the 9234 1451 224 first-chance fission fitting without modification, we performed 9234 1451 225 GNASH calculations over the entire energy region of each target 9234 1451 226 nucleus. We carried the calculations to 30 MeV, which involve 9234 1451 227 first-, second-, third-, fourth-, and fifth-chance fission 9234 1451 228 processes. These comparisons provide a necessary test of the 9234 1451 229 reliability of our calculations, in that no adjustments are made 9234 1451 230 past the first-chance fission results. 9234 1451 231 9234 1451 232 III. DESCRIPTION OF EVALUATED DATA BASE 9234 1451 233 9234 1451 234 A. Total Cross Section 9234 1451 235 9234 1451 236 The evaluated total cross section below 10 keV is obtained 9234 1451 237 from the resonance parameter evaluation in ENDF/B-VI, with the 9234 1451 238 fission channel modified as described below. From 10 keV to 30 9234 1451 239 MeV, the coupled-channel deformed optical model calculations 9234 1451 240 described above are used directly. 9234 1451 241 9234 1451 242 B. Elastic Cross Section 9234 1451 243 9234 1451 244 The elastic cross section at all energies is obtained from 9234 1451 245 the difference of the total and nonelastic cross sections. 9234 1451 246 Below 10 keV it comes from the modified ENDF/B-VI resonance 9234 1451 247 parameters and at higher energies it is determined by the 9234 1451 248 coupled-channel optical model calculations. Angular 9234 1451 249 distributions for elastic neutrons were obtained at all energies 9234 1451 250 from earlier (Yo94) coupled-channel calculations and are given 9234 1451 251 as Legendre expansions. 9234 1451 252 9234 1451 253 C. Fission Cross Section 9234 1451 254 9234 1451 255 The background present in the resolved resonance region 9234 1451 256 (below 102.5 eV) was lowered to improve agreement with a limit 9234 1451 257 given for the thermal fission cross section by Mughabghab 9234 1451 258 (Mu84). At higher energies the fission cross section is based 9234 1451 259 on the theoretical analysis described above. 9234 1451 260 9234 1451 261 D. Radiative Capture Cross Section 9234 1451 262 9234 1451 263 Below 10 keV, the capture cross section is based on the 9234 1451 264 ENDF/B-VI resonance parameters. At higher energies the cross 9234 1451 265 section is calculated using the generalized Lorentzian model of 9234 1451 266 Ko90. The normalization of the strength function was set by 9234 1451 267 requiring the calculated (n,g) cross section be consistent with 9234 1451 268 measured values for 235U. 9234 1451 269 9234 1451 270 E. Inelastic Neutron Cross Sections 9234 1451 271 9234 1451 272 Discrete (n,n') cross sections are included for the lowest 25 9234 1451 273 excited states of 237U. The first and second excited states are 9234 1451 274 members of the K = 1/2 ground-state rotational band and include 9234 1451 275 coupled-channel as well as compound nucleus contributions. The 9234 1451 276 remaining discrete-state cross sections through the 25th excited 9234 1451 277 state are based on compound nucleus calculations with 9234 1451 278 preequilibrium corrections with the GNASH code. Angular 9234 1451 279 distributions for the discrete inelastic neutrons are taken from 9234 1451 280 the earlier [Yo94] analysis. 9234 1451 281 The inelastic data corresponding to excitation energies in 9234 1451 282 237U above 0.54 MeV are given as energy-angle correlated 9234 1451 283 continuous spectra and were calculated with the GNASH code. The 9234 1451 284 results are given in File 6 of the ENDF/B-formatted evaluation 9234 1451 285 (ENDF-6 format) and utilize systematics by Kalbach (Ka88) for 9234 1451 286 angular distribution information, parameterized in terms of 9234 1451 287 preequilibrium ratios calculated in GNASH. 9234 1451 288 The total inelastic neutron cross section from the present 9234 1451 289 analysis is drastically different from ENDF/B-VI in the energy 9234 1451 290 range below a few MeV. Additionally, it should be pointed out 9234 1451 291 that the emission spectrum of inelastic neutrons is also 9234 1451 292 drastically different because it is dominated at lower energies 9234 1451 293 by direct reaction effects, which were apparently not included 9234 1451 294 in the ENDF/B-VI evaluation. 9234 1451 295 9234 1451 296 F. Cross Sections for 237U(n,xn) Reactions 9234 1451 297 9234 1451 298 The 237U(n,2n), (n,3n), and (n,4n) cross sections result 9234 1451 299 entirely from the theoretical analysis and GNASH calculations. 9234 1451 300 The present analysis is somewhat similar to ENDF/B-VI below 12 9234 1451 301 MeV but is significantly different near 14 MeV. The (n,3n) and 9234 1451 302 (n,4n) cross sections are also significantly different from 9234 1451 303 ENDF/B-VI near 14 MeV. 9234 1451 304 Energy-angle correlated distributions are given for all the 9234 1451 305 237U(n,xn) reactions, making use of Kalbach's systematics (Ka88) 9234 1451 306 and the ENDF/B-6 File 6 representation. 9234 1451 307 9234 1451 308 G. Nubar 9234 1451 309 9234 1451 310 The evaluation of delayed and prompt nubar were carried over 9234 1451 311 directly from the ENDF/B-VI evaluation of 237U. The prompt 9234 1451 312 nubar evaluation is based on the systematics of Manero and 9234 1451 313 Konshin (Ma72). 9234 1451 314 9234 1451 315 H. Fission Neutron Spectra 9234 1451 316 9234 1451 317 The fission neutron spectra in the revised evaluation is also 9234 1451 318 carried over directly from the 237U evaluation in ENDF/B-VI. A 9234 1451 319 maxwellian representation is used for the spectrum shape, with 9234 1451 320 energy-dependent temperature parameters based on systematics. 9234 1451 321 9234 1451 322 9234 1451 323 IV. CONCLUSIONS 9234 1451 324 9234 1451 325 The new analysis of n + 237U nuclear data should provide a 9234 1451 326 much improved representation of most reactions over the incident 9234 1451 327 energy range 10 keV to 30 MeV. The most significant and obvious 9234 1451 328 improvement is in the inelastic neutron cross sections, spectra, 9234 1451 329 and angular distributions in the energy range from threshold to 9234 1451 330 5 MeV. The fission cross section was reevaluated using model 9234 1451 331 parameters consistent with neighboring U isotopes. The new 9234 1451 332 analysis also should result in improved representations of the 9234 1451 333 (n,xn) cross sections, and certainly in the (n,xn) neutron 9234 1451 334 energy and angular distributions. 9234 1451 335 This evaluation is regarded as preliminary until the results 9234 1451 336 of our assumptions regarding the fission cross section can be 9234 1451 337 assessed in integral calculations. Additionally, improvements 9234 1451 338 to the evaluations of nubar and the fission neutron spectra 9234 1451 339 using the Madland-Nix approach will be considered in the future. 9234 1451 340 9234 1451 341 **************************************************************** 9234 1451 342 9234 1451 343 REFERENCES 9234 1451 344 9234 1451 345 Ar82a E. D. Arthur, "Use of the Statistical Model for the 9234 1451 346 Calculation of Compound Nucleus Contributions to Inelastic 9234 1451 347 Scattering on Actinide Nuclei," Proc. of OECD/NEA Specialists' 9234 1451 348 Meeting on Fast Neutron Scattering on Actinide Nuclei, (Paris, 9234 1451 349 November, 1981), NEANDC-158 "U" (1982) p. 145. 9234 1451 350 9234 1451 351 Ar82b E. D. Arthur, "Use of Fission Probability Data in the 9234 1451 352 Calculation of n + 237U Fission Cross Sections," in Applied 9234 1451 353 Nuclear Data Research and Development: April 1, 1982 - Setember 9234 1451 354 30, 1982 (Cp. E. D. Arthur) LA-9647-PR (1982) p. 24. 9234 1451 355 9234 1451 356 Ar82c E. D. Arthur, "An Improved Method for Use of Measured 9234 1451 357 Fission Probabilities in Neutron Fission Cross-Section 9234 1451 358 Determination," in Applied Nuclear Data Research and 9234 1451 359 Development: April 1, 1982 - Setember 30, 1982 (Cp. E. D. 9234 1451 360 Arthur) LA-9647-PR (1982) p. 19. 9234 1451 361 9234 1451 362 Ba74 B. B. Back, O. Hansen, H. C. Britt, and J. D. Garrett, 9234 1451 363 "Fission of Doubly Even Actinide Nuclei Induced by Direct 9234 1451 364 Reactions, " Phys. Rev. C 9, 1924 (1974). 9234 1451 365 9234 1451 366 Br82 H. C. Britt, personal communication, 1982. 9234 1451 367 9234 1451 368 Cr70 J. D. Cramer and H. C. Britt, "Neutron Fission Cross 9234 1451 369 Sections for 231Th, 233Th, 235U, 237U, 239U, 241Pu, and 243Pu 9234 1451 370 from 0.5 to 2.25 MeV Using (t,pf) Reactions," Nucl. Sci. Engr. 9234 1451 371 41, 177 (1970). 9234 1451 372 9234 1451 373 Du70 C. L. Dunford, "A Unified Model for Analysis of Compound 9234 1451 374 Nucleus Reactions,"AI-AEC-12931, Atomics Int. (1970). 9234 1451 375 9234 1451 376 Gi65 A. Gilbert and A. G. W. Cameron, "A Composite Nuclear- 9234 1451 377 Level Density Formula with Shell Corrections," Can. J. Phys. 43, 9234 1451 378 1446 (1965). 9234 1451 379 9234 1451 380 Ha82 G. Haouat, J. Lachkar, Ch. Lagrange, J. Jary, J. Sigaud, 9234 1451 381 and Y. Patin, "Neutron Scattering Cross Sections for 232Th, 9234 1451 382 233U, 235U, 238U, 239Pu, and 242Pu Between 0.6 and 3.4 MeV," 9234 1451 383 Nucl. Sci. and Engr. 81, 491 (1982). 9234 1451 384 9234 1451 385 Ja75 J. Jary, "Methode de Calcul par Modele Statistique des 9234 1451 386 Sections Efficaces des Reactions (n,xn) et (n,xnf) Pour les 9234 1451 387 Isotopes de l'Uranium 232U a 239U dans le Domaine d'Energie 2 9234 1451 388 MeV - 15 MeV," Commissariat a l'Energie Atomique Report CEA-R- 9234 1451 389 4647 (1975). 9234 1451 390 9234 1451 391 Ka88 C. Kalbach, "Systematics of Continuum Angular 9234 1451 392 Distributions: Extensions to Higher Energies," Phys. Rev. C37, 9234 1451 393 2350 (1988); C. Kalbach and F. M. Mann, "Phenomenology of 9234 1451 394 Continuum Angular Distributions. I. Systematics and 9234 1451 395 Parameterization," Phys. Rev. C 23, 112 (1981). 9234 1451 396 9234 1451 397 Ko90 J. Kopecky and M.Uhl, "Test of Gamma-Ray Strength 9234 1451 398 Functions in Nuclear Reaction Model Calculations," Phys. Rev. C 9234 1451 399 42, 1941 (1990). 9234 1451 400 9234 1451 401 Ma72 F. Manero and V. A. Konshin, At. En. Rev. 10, 637 (1972). 9234 1451 402 9234 1451 403 Ma78 D. G. Madland and P. G. Young, "Neutron-Nucleus Optical 9234 1451 404 Potential for the Actinide Region," Proc. Int. Conf. on Neutron 9234 1451 405 Physics and Nuclear Data for Reactors and Other Applied 9234 1451 406 Purposes, Harwell, England (pub. by OECD), p. 349 (1978). 9234 1451 407 9234 1451 408 Mc74 J. H. McNally, J. W. Barnes, B. J. Dropesky, P. A. Seeger 9234 1451 409 and K. Wolfsberg, "Neutron-Induced Fission Cross Section of 9234 1451 410 237U," Phys. Rev. C 9, 717 (1974). 9234 1451 411 9234 1451 412 Mo95 P. Moller, J. R. Nix, W. D. Myers, and W. J. Swiatecki, 9234 1451 413 "Ground-State Masses and Deformations," Atomic Data Nucl. Data 9234 1451 414 Tables 59 (1995),1. 9234 1451 415 9234 1451 416 Mu84 S. F. Mughabghab, in Neutron Cross Sections, Vol. 1, 9234 1451 417 "Neutron Resonance Parameters and Thermal Cross Sections," Part 9234 1451 418 B, Z = 61-100, Academic Press, New York (1984). 9234 1451 419 9234 1451 420 Ra70 J. Raynal, "Optical-Model and Coupled-Channel Calculations 9234 1451 421 in Nuclear Physics," IAEA SMR-9/8, Int. At. En. Agency (1970). 9234 1451 422 9234 1451 423 Yo88 P. G. Young and E. D. Arthur, "Calculation of 235U(n,n') 9234 1451 424 Cross Sections for ENDF/B-VI," Int. Conf. on Nucl. Data for 9234 1451 425 Science and Technology, Mito, Japan, May 30 - June 3, 1988 (Ed. 9234 1451 426 S. Igarasi, Saikon Publ. Co., Ltd., 1988) p. 603. 9234 1451 427 9234 1451 428 Yo92a P. G. Young and E. D. Arthur, "Theoretical Analyses of 9234 1451 429 (n,xn) Reactions on 235U, 238U, 237Np, and 239Pu for ENDF/B-VI," 9234 1451 430 Proc. Int. Conf. on Nuclear Data for Science and Technology, 9234 1451 431 Julich, Germany, 13-17 May 1991 (LA-UR-91-1424), [Ed. S. M. 9234 1451 432 Qaim, Springer-Verlag, Germany (1992)], p. 894. 9234 1451 433 9234 1451 434 Yo92b P. G. Young, E. D. Arthur, and M. B. Chadwick, 9234 1451 435 "Comprehensive Nuclear Model Calculations: Introduction to the 9234 1451 436 Theory and Use of the GNASH Code," Los Alamos National 9234 1451 437 Laboratory report LA-12343-MS (1992). 9234 1451 438 9234 1451 439 Yo94 P. G. Young, "Preliminary Evaluation of n + 237U 9234 1451 440 Reactions," Los Alamos National Laboratory internal memo #T-2: 9234 1451 441 M-3669 (P. G. Young to R. C. Little, 3 February 1994). 9234 1451 442 9234 1451 443 ******************************************************************9234 1451 444 THE DESCRIPTION BELOW IS TAKEN FROM THE ENDF/B-VI.2 FILE. 9234 1451 445 IT DESCRIBES THE MF=1 (NUBAR) AND MF=2 (RESONANCE PARAMETER) DATA.9234 1451 446 ******************************************************************9234 1451 447 9234 1451 448 ENDF/B-VI REVISION 1 9234 1451 449 ADDED MISSING FISSION NEUTRON ANGULAR DISTRIBUTION MF=4 MT=18 9234 1451 450 ASSUMED TO BE ISOTROPIC 9234 1451 451 ******************************************************************9234 1451 452 ENDF/B-V MATERIAL CONVERTED TO ENDF-6 FORMAT BY NNDC 9234 1451 453 * * * * * * *9234 1451 454 THIS EVALUATION IS A COMBINATION OF THE EVALUATION OF BENJAMIN 9234 1451 455 AND MCCROSSON AT SRL AND THE ENDL EVALUATION OF HOWERTON (REF.5).9234 1451 456 BOTH SOURCES WERE MODIFIED TO CONFORM TO THE ENDF/B-V FORMAT 9234 1451 457 SPECIFICATIONS. IMPORTANT CHANGES OR MODIFICATIONS ARE NOTED. 9234 1451 458 MF=1 GENERAL INFORMATION 9234 1451 459 MT=452 NUBAR THERMAL VALUE COMPUTED FROM SEMI-EMPIRICAL WORK 9234 1451 460 OF GORDEEVA AND SMIRENKIN(REF.1) AS REVISED BY MANERO AND 9234 1451 461 KONSHIN(REF.2). ENERGY DEPENDENCE BASED ON WORK OF HOWER- 9234 1451 462 TON(REF.5). RENORMALIZATION OF HOWERTON SHAPE DONE AT BNL. 9234 1451 463 MT=455 DEL. NUBAR, M.C.BRADY+T.R.ENGLAND, NSE 103,129(1989) 9234 1451 464 MF=2 RESONANCE PARAMETERS 9234 1451 465 MT=151 RESOLVED RESONANCES RESONANCE PARAMETERS DETERMINED BY 9234 1451 466 THE GENRPAR CODE(REF.3) BASED UPON THE SRL DATA SET AND AN 9234 1451 467 AVERAGE LEVEL SPACING OF 3.5 EV(REF.4). RESOLVED REGION- 9234 1451 468 0 TO 102.5 EV. 9234 1451 469 NOTE: A BOUND LEVEL AT -2.109 EV WAS REMOVED FROM THE SRL 9234 1451 470 PARAMETERS AND APPROPRIATE BACKGROUNDS WERE INSERTED INTO THE9234 1451 471 TOT, NF, AND NG FILES (MF=3, MT=1,18,102). 9234 1451 472 * * * * * * 9234 1451 473 UNRESOLVED RESONANCES SAME BASIS AS RESOLVED, WITH 9234 1451 474 AVERAGE RESONANCE PARAMETERS. UNRESOLVED REGION - 102.5 EV 9234 1451 475 TO 10 KEV. 9234 1451 476 ******************************************************************9234 1451 477 Note that MF=8,12,13,14,15 were also taken over directly from 9234 1451 478 ENDF/B-VI. The gamma production data are from an LLNL evaluation.9234 1451 479 ******************************************************************9234 1451 480 1 451 566 39234 1451 481 1 452 10 09234 1451 482 1 455 7 39234 1451 483 1 456 8 09234 1451 484 1 458 11 19234 1451 485 2 151 202 09234 1451 486 3 1 42 39234 1451 487 3 2 42 39234 1451 488 3 3 42 39234 1451 489 3 4 27 39234 1451 490 3 16 18 39234 1451 491 3 17 14 39234 1451 492 3 18 31 39234 1451 493 3 37 9 39234 1451 494 3 51 27 39234 1451 495 3 52 26 39234 1451 496 3 53 26 39234 1451 497 3 54 26 39234 1451 498 3 55 25 39234 1451 499 3 56 25 39234 1451 500 3 57 25 39234 1451 501 3 58 24 39234 1451 502 3 59 24 39234 1451 503 3 60 24 39234 1451 504 3 61 23 39234 1451 505 3 62 23 39234 1451 506 3 63 23 39234 1451 507 3 64 22 39234 1451 508 3 65 22 39234 1451 509 3 66 22 39234 1451 510 3 67 21 39234 1451 511 3 68 21 39234 1451 512 3 69 21 39234 1451 513 3 70 20 39234 1451 514 3 71 20 39234 1451 515 3 72 20 39234 1451 516 3 73 19 39234 1451 517 3 74 19 39234 1451 518 3 75 18 39234 1451 519 3 91 18 39234 1451 520 3 102 26 39234 1451 521 4 2 101 39234 1451 522 4 18 2 39234 1451 523 4 51 99 39234 1451 524 4 52 97 39234 1451 525 4 53 97 39234 1451 526 4 54 50 39234 1451 527 4 55 97 39234 1451 528 4 56 48 39234 1451 529 4 57 95 39234 1451 530 4 58 48 39234 1451 531 4 59 48 39234 1451 532 4 60 48 39234 1451 533 4 61 48 39234 1451 534 4 62 48 39234 1451 535 4 63 48 39234 1451 536 4 64 48 39234 1451 537 4 65 48 39234 1451 538 4 66 48 39234 1451 539 4 67 48 39234 1451 540 4 68 48 39234 1451 541 4 69 48 39234 1451 542 4 70 48 39234 1451 543 4 71 48 39234 1451 544 4 72 48 39234 1451 545 4 73 46 39234 1451 546 4 74 46 39234 1451 547 4 75 46 39234 1451 548 5 18 9 39234 1451 549 5 455 589 39234 1451 550 6 16 1486 39234 1451 551 6 17 738 39234 1451 552 6 37 392 39234 1451 553 6 91 2552 39234 1451 554 8 16 2 39234 1451 555 8 17 2 39234 1451 556 8 102 2 39234 1451 557 12 18 4 39234 1451 558 12 102 4 39234 1451 559 13 3 11 39234 1451 560 14 3 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0 0 1 49234 1455 4 4 2 9234 1455 5 1.000000-5 3.495967-2 4.000000+6 3.495967-2 7.000000+6 2.097580-29234 1455 6 3.000000+7 2.097580-2 9234 1455 7 0.000000+0 0.000000+0 0 0 0 09234 1 099999 9.223700+4 2.350124+2 0 2 0 09234 1456 1 0.000000+0 0.000000+0 0 0 1 159234 1456 2 15 2 9234 1456 3 1.000000-5 2.395040+0 4.000000+6 2.971650+0 5.000000+6 3.117470+09234 1456 4 6.000000+6 3.370900+0 7.000000+6 3.593130+0 8.000000+6 3.747580+09234 1456 5 9.000000+6 3.891730+0 1.000000+7 4.015290+0 1.100000+7 4.159440+09234 1456 6 1.200000+7 4.344780+0 1.300000+7 4.519830+0 1.400000+7 4.561010+09234 1456 7 1.460000+7 4.736050+0 2.000000+7 5.436220+0 3.000000+7 6.732831+09234 1456 8 0.000000+0 0.000000+0 0 0 0 09234 1 099999 9.223700+4 2.350124+2 0 0 0 09234 1458 1 0.000000+0 0.000000+0 0 2 54 279234 1458 2 1.693413+8 9.313774+6 4.948000+6 4.800000+4 1.927000+4 1.253000+39234 1458 3 7.229954+6 7.229954+4 3.097368+6 1.584602+4 3.185049+6 1.056401+49234 1458 4 4.281593+6 1.584602+4 1.878210+8 1.624876+7 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