$Rev:: 532 $ $Date:: 2011-12-05#$ 1 0 0 0 9.424100+4 2.389780+2 1 1 0 19443 1451 1 0.000000+0 1.000000+0 0 0 0 69443 1451 2 1.000000+0 2.000000+7 1 0 10 79443 1451 3 0.000000+0 0.000000+0 0 0 440 729443 1451 4 94-Pu-241 ORNL EVAL-OCT03 L.Weston,R.Wright,H.Derrien + 9443 1451 5 DIST-SEP10 20111222 9443 1451 6 ----ENDF/B-VII.1 MATERIAL 9443 9443 1451 7 -----INCIDENT NEUTRON DATA 9443 1451 8 ------ENDF-6 FORMAT 9443 1451 9 9443 1451 10 ----------------------------------------------------------------- 9443 1451 11 ENDF/A: Fission Cross Section Covariance Matrix Added 9443 1451 12 ----------------------------------------------------------------- 9443 1451 13 P.G.Young, P.Talou 9443 1451 14 Los Alamos National Laboratory, March 2010 9443 1451 15 9443 1451 16 A covariance analysis of experimental fission cross section data 9443 1451 17 sets from 1 keV up to 30 MeV was performed with the GLUCS code. 9443 1451 18 It is based on 13 data sets, including the most recent shape 9443 1451 19 measurement by Tovesson at LANSCE, Los Alamos. However, 9443 1451 20 discrepancies below 0.9 MeV between Tovesson data and a majority 9443 1451 21 of other data sets led us to discard the LANSCE data below this 9443 1451 22 point. This is only a temporary solution, as we thrive to better 9443 1451 23 understand the observed discrepancies. Some other data sets were 9443 1451 24 also discarded, due to very large assumed uncertainties. Finally, 9443 1451 25 a systematic error of 1.5% was added to the diagonal elements, 9443 1451 26 while keeping the correlation matrix unchanged. Future work should9443 1451 27 lead to a better justification for this additional contribution. 9443 1451 28 A new section MF33, MT18 has been added to the ENDF/B-VII.0 file. 9443 1451 29 This is only a preliminary result, as more work is expected to 9443 1451 30 perform a complete new evaluation, including covariance work, in 9443 1451 31 the next year. 9443 1451 32 Covariances in the thermal and resonance region are based on 9443 1451 33 revisited low-fidelity estimates. 9443 1451 34 9443 1451 35 FEBRUARY 28 2003 9443 1451 36 ---------------------------------------------------------------- 9443 1451 37 Reevaluation of rhe resonance parameters in the energy range up 9443 1451 38 to 20 eV - Colaboration ORNL(USA)-CEN/CAD(FRANCE) 9443 1451 39 H. Derrien and L.C Leal, ORNL 9443 1451 40 A. Courcelle and A. Santamarina, CEN/CAD 9443 1451 41 (submitted to NSE, 2003) 9443 1451 42 9443 1451 43 9443 1451 44 Cross section integrals in the energy range 0.0021 eV to 20.0 eV 9443 1451 45 9443 1451 46 ------------------------------------------------------------- 9443 1451 47 Energy Range Capture b-eV Fission b-eV 9443 1451 48 eV 1993 Present 1993 Present 9443 1451 49 ------------------------------------------------------------- 9443 1451 50 0.0021-0.020 12.25 12.51 2.1% 31.06 31.43 1.2% 9443 1451 51 0.0200-0.030 3.67 3.72 1.4% 10.24 10.36 1.2% 9443 1451 52 0.0300-0.100 15.28 15.59 2.0% 49.02 49.14 0.2% 9443 1451 53 0.1000-0.500 110.58 117.40 6.2% 262.76 263.84 0.4% 9443 1451 54 0.5000-1.000 5.90 6.03 2.2% 17.93 17.89 -0.2% 9443 1451 55 1.0000-3.000 7.30 7.16 -2.0% 54.88 52.89 -3.8% 9443 1451 56 3.0000-20.00 1213. 1234. 1.7% 3039. 3026. -0.4% 9443 1451 57 ------------------------------------------------------------- 9443 1451 58 9443 1451 59 The cross sections at 0.0253 eV are the following: 9443 1451 60 9443 1451 61 Total 1386.5 b 9443 1451 62 Fission 1012.2 b 9443 1451 63 Capture 363.0 b 9443 1451 64 9443 1451 65 very close to the current standard. 9443 1451 66 9443 1451 67 The fit of the experimental data (Young total, Wagemans fission, 9443 1451 68 Weston capture and Weston fission ) were performed by assuming 9443 1451 69 that young total and Wagemans fission were OK with the standard 9443 1451 70 and that Weston original data(from the EXFOR file)needed a renor- 9443 1451 71 zation to agree with the standard. A consistent normalization 9443 1451 72 was obtained by a SAMMY fit leading to a decrease of 4.5% 9443 1451 73 in the original Weston fission and a decrease of 3.0% in the 9443 1451 74 original Weston capture.The differences between the 1988, 1993 9443 1451 75 and the present results are consistent with the experimental 9443 1451 76 errors given by Weston for the measured fission (2-3%) and 9443 1451 77 capture (10-15%). The default of normalization of the Weston 9443 1451 78 fission,due to severe experimental errors in the thermal range, 9443 1451 79 was responsible for the large uncertainty in the capture results. 9443 1451 80 9443 1451 81 9443 1451 82 9443 1451 83 9443 1451 84 ***************************************************************** 9443 1451 85 * * * * * 9443 1451 86 CHANGES FOR REVISION 2 WERE INSERTION OF REVISED RESONANCE REGION9443 1451 87 PARAMETERS BY DERRIEN; RENORMALIZATION OF CAPTURE ABOVE THE 9443 1451 88 RESOLVED RESONANCE REGION TO BE 4.8% LOWER THAN VERSION 5 AND 9443 1451 89 UPWARD FROM 14% DOWN IN ORIGINAL VERSION 6. SCATTERING WAS 9443 1451 90 ADJUSTED TO MAKE UP DIFFERENCE. THE RENORMALIZATION WAS THE 9443 1451 91 SUGGESTION OF DERRIEN AFTER STUDY OF THE NEW MEASUREMENTS BY 9443 1451 92 WAGEMANS ET AL., REF 1. 9443 1451 93 * * * * * 9443 1451 94 PU-241 WAS REVISED FOR VERSION VI BY L.W.WESTON. THE 9443 1451 95 CHANGES WERE THE ADOPTION OF THE RECOMMENDED VALUES OF THE 9443 1451 96 STANDARDS COMMITTEE FOR THE THERMAL CONSTANTS; THE ADOPTION 9443 1451 97 OF THE REICH-MOORE RESONANCE PARAMETER EVALUATION OF THE 9443 1451 98 RESOLVED RESONANCE REGION BY H.DERRIEN,REF 2., OF CADARACHE, 9443 1451 99 FRANCE; RENORMALIZATION OF CAPTURE ABOVE 300EV BY 14% DOWNWARD 9443 1451 100 AS RECOMMENDED BY H.DERRIEN. THE TOTALS ABOVE 100 KEV WERE MADE 9443 1451 101 SAME AS PU-239. CAPTURE REVISED DOWNWARD ABOVE 1.5 MEV. 9443 1451 102 COVARIANCES WERE STRIPED OFF BECAUSE THEY WERE DEPENDANT ON 9443 1451 103 U-235 COVARIANCES WHICH ARE NOT COMPLETED. 9443 1451 104 ******************************************************************9443 1451 105 MF=1 MT=452 THERMAL NUBAR OF 2.9453 RECOMMENDED BY STANDARDS 9443 1451 106 COMMITTEE. PROMPT RATIOS TO CF ABOVE .47 MEV FROM 9443 1451 107 FREHAUT,REF.3. NUBAR PROMPT OF CF OF 3.7676. 9443 1451 108 MF=1 MT=455 TABULATION OF NU DELAYED (REF.4) EXCEPT THERMAL. 9443 1451 109 MF=1 MT=456 SEE MT=452 9443 1451 110 MF=2 MT=151 RESOLVED RESONANCE REGION 10-5 TO 300EV,REICH-MOORE 9443 1451 111 $$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$9443 1451 112 REVISED RESONANCE DATA ,JAERI MAY 1993 9443 1451 113 ***************************************************************** 9443 1451 114 Revision of the 241Pu Reich-Moore resonance parameters 9443 1451 115 by comparison with recent fission cross section measurements. 9443 1451 116 9443 1451 117 Herve Derrien 9443 1451 118 Japanese Atomic Energy Research Institute 9443 1451 119 9443 1451 120 I-INTRODUCTION. 9443 1451 121 The resonance parameters of the neutron cross sections 9443 1451 122 of 241Pu were obtained by Derrien and de Saussure(2) in the energy9443 1451 123 range from thermal to 300 eV by a Bayesian fit of selected 9443 1451 124 experimental effective total cross sections, fission and capture 9443 1451 125 cross sections by using the Reich-Moore fitting code SAMMY(5). 9443 1451 126 The results of this work were used in the ENDF/B-VI evaluated data9443 1451 127 file. Some difficulties were encountered in the normalization of 9443 1451 128 the experimental fission cross sections due to the discrepancies 9443 1451 129 in the shape of the available experimental data both in thermal 9443 1451 130 and high energy ranges. The consistency among the experimental 9443 1451 131 data base could not be obtained without large renormalization and 9443 1451 132 background correction parameters in the SAMMY fits. Particularly,9443 1451 133 it was shown that the discrepancy between the fission cross 9443 1451 134 sections in the thermal energy range was due to a deviation from 9443 1451 135 the 1/v shape below about 0.05 eV. 9443 1451 136 New fission cross section measurements were recently 9443 1451 137 performed by Wagemans et al.(1,6) in the energy range from 0.002 9443 1451 138 eV to 20 eV in order to check the shape of the cross section in 9443 1451 139 the thermal energy range. They showed that the shape of the 9443 1451 140 fission cross section was clearly compatible with the 1/v law,in 9443 1451 141 contradiction to all the previous measurements reported in the 9443 1451 142 literature. Consequently, the normalization of all the 9443 1451 143 previous results using the low energy region could be erroneous. 9443 1451 144 Particularly,the discrepancy observed in the average fission 9443 1451 145 cross section over the 0.26 eV resonance could be due to the 9443 1451 146 errors of normalization in the thermal region. Wagemans et al. 9443 1451 147 compared the ENDF/B-VI data to their new results and concluded 9443 1451 148 that the evaluated data files using the evaluation of Derrien and 9443 1451 149 de Saussure should be revised in the energy range up to 300 eV. 9443 1451 150 9443 1451 151 II-COMMENTS ON ENDF/B-VI EVALUATION. 9443 1451 152 9443 1451 153 In the energy range from 0.01 eV to 3 eV the new data of 9443 1451 154 Wagemans et al. are on average 2.2% smaller than ENDF/B-VI. This 9443 1451 155 difference is mainly due a difference of 3% between the 1976 data 9443 1451 156 of Wagemans et al.(7) and the new values of Wagemans et al. The 9443 1451 157 1976 data of Wagemans et al. were used in the evaluation of 9443 1451 158 Derrien and de Saussure in the low energy region. 9443 1451 159 In the intermediate energy range from 3 eV to 12 eV,the 9443 1451 160 average fission of ENDF/B-VI is in excellent agreement with the 9443 1451 161 new data of Wagemans et al. In this energy range,the SAMMY fits of9443 1451 162 Derrien and de Saussure were performed on the fission cross 9443 1451 163 section of Weston and Todd(8),of Blons(9) and of Migneco et al. 9443 1451 164 (10) with an adjustment of the normalization factor and of the 9443 1451 165 background correction parameters of all the experimental data; the9443 1451 166 agreement between the new data of Wagemans et al. and ENDF/B-VI 9443 1451 167 shows that, at least in this energy range, SAMMY performed on the 9443 1451 168 data of Weston and Todd a renormalization equivalent to that 9443 1451 169 recommended by Wagemans et al.(1). 9443 1451 170 In the higher range up to 300 eV,the SAMMY fits relied 9443 1451 171 mainly on the high resolution measurements of Blons and of 9443 1451 172 Migneco et al. for the accurate determination of the resonance 9443 1451 173 parameters. Quite large normalization coefficients and background9443 1451 174 correction parameters were also needed in this energy range to 9443 1451 175 obtain the consistency between the calculated cross sections and 9443 1451 176 the experimental data. However,the result of the fits was in quite9443 1451 177 good agreement with the data of Weston and Todd normalized to the 9443 1451 178 1976 data of Wagemans et al.in the low energy region, which is 9443 1451 179 also equivalent to the normalization to the 1983 data of Wagemans 9443 1451 180 et al.(11). Since the earlier data of Wagemans et al. should 9443 1451 181 decrease by 3% to be consistent with the new data, it is likely 9443 1451 182 that the ENDF/B-VI fission cross section could be too large by 9443 1451 183 about 3% in the energy range above 12 eV. 9443 1451 184 9443 1451 185 III-REVISION OF THE RESONANCE PARAMETERS. 9443 1451 186 9443 1451 187 An accurate up-dating of the 241Pu resonance parameters 9443 1451 188 could be obtained by renormalizing the fission experimental data 9443 1451 189 base according to the new data of Wagemans et al. and by 9443 1451 190 restarting the SAMMY fits of the new experimental data base, 9443 1451 191 including the high resolution transmission data of Harvey and 9443 1451 192 Simpson(12). Due to lack of time a new SAMMY analysis was 9443 1451 193 performed only in the energy range from 0.002 eV to 3 eV. In the 9443 1451 194 energy range above 3 eV the up-dating was performed by applying 9443 1451 195 some small corrections to the resonance parameters. 9443 1451 196 The SAMMY analysis of the new Wagemans et al. data was 9443 1451 197 performed along with the total cross section of Young and 9443 1451 198 Smith(13) in the energy range from 0.002 eV to 3 eV,by starting 9443 1451 199 with the ENDF/B-VI resonance parameters. Only the parameters of 9443 1451 200 the 3+ resonances at -0.122 eV and at 0.265 eV were adjusted in 9443 1451 201 this energy range. The values of the cross sections calculated 9443 1451 202 at 0.0253 eV are compared to the standard data(14) in Table 1. The9443 1451 203 average total,fission and capture cross sections calculated with 9443 1451 204 the new resonance parameters are displayed on Table 2,3 and 4 with9443 1451 205 the corresponding experimental data and the values obtained from 9443 1451 206 ENDF/B-VI. One should point out that an energy shift of 9443 1451 207 dE/E=+0.00384 was applied to the data of Young and Smith in order 9443 1451 208 to achieve a good consistency with the energy scale of the 9443 1451 209 fission data of Wagemans et al. over the resonance at 0.0265 eV. 9443 1451 210 In the energy range above 3 eV the small corrections 9443 1451 211 applied to the resonance parameters result in a decrease of the 9443 1451 212 average fission cross section and in an increase of the average 9443 1451 213 capture cross section,with a variation of the average total cross 9443 1451 214 section smaller than the errors of the experimental data of Harvey9443 1451 215 and Simpson. The average values of the fission and capture cross 9443 1451 216 sections calculated with the new resonance parameters are shown in9443 1451 217 Table 5 and 6 along with the renormalized fission cross section of9443 1451 218 Weston and Todd and the values calculated from ENDF/B-VI. 9443 1451 219 9443 1451 220 IV-CONCLUSION. 9443 1451 221 9443 1451 222 The results of the recent measurement of the 241Pu fission9443 1451 223 cross section in the energy range from 0.002 eV to 4 eV of 9443 1451 224 Wagemans et al. were used in a new evaluation of the resonance 9443 1451 225 parameters. The accuracy of the calculated cross sections was 9443 1451 226 greatly improved in the resonance at 0.265 eV. The cross sections 9443 1451 227 averaged over this resonance should have the same accuracy as 9443 1451 228 the standard values at 0.0253 eV. In the high energy region up 9443 1451 229 to 300 eV the SAMMY analysis of the new experimental data base 9443 1451 230 obtained by the renormalization of the experimental data is 9443 1451 231 recommended in order to improve the corrections to the resonance 9443 1451 232 parameters performed in the present work. 9443 1451 233 9443 1451 234 9443 1451 235 Table 1 9443 1451 236 9443 1451 237 Cross sections at 0.0253 eV 9443 1451 238 9443 1451 239 ------------------------------------------------------------- 9443 1451 240 Present results ENDF/B-VI Standard(14) 9443 1451 241 ------------------------------------------------------------- 9443 1451 242 Fission 1012.50(-0.0%) 1012.68+-6.58 9443 1451 243 Capture 361.52(+0.1%) 361.29+-4.95 9443 1451 244 Scattering 11.36(-7.1%) 12.17+-2.62 9443 1451 245 Total 1385.38(-0.1%) 1386.14+-8.64 9443 1451 246 ------------------------------------------------------------- 9443 1451 247 9443 1451 248 9443 1451 249 Table 2 9443 1451 250 9443 1451 251 The total cross section integral in the energy range from 9443 1451 252 0.0021 eV to 3 eV. 9443 1451 253 9443 1451 254 ------------------------------------------------------------------9443 1451 255 Energy range Present work ENDF/B-VI Young and Smith(13) 9443 1451 256 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 257 ------------------------------------------------------------------9443 1451 258 0.0021-0.020 43.54 43.09(-1.0%) 43.25(-0.7%) 9443 1451 259 0.0200-0.030 14.03 14.02(-0.1%) 14.01(-0.1%) 9443 1451 260 0.0300-0.100 65.09 66.17(+1.7%) 64.99(-0.1%) 9443 1451 261 0.1000-0.500 378.38 385.27(+1.8%) 380.10(+0.4%) 9443 1451 262 0.5000-1.000 29.74 29.41(-1.1%) 31.19(+4.4%) 9443 1451 263 1.0000-3.000 83.36 83.92(+0.7%) 82.50(-1.0%) 9443 1451 264 ------------------------------------------------------------------9443 1451 265 0.0021-3.000 614.14 621.88(+1.3%) 616.04(+0.3%) 9443 1451 266 ------------------------------------------------------------------9443 1451 267 9443 1451 268 9443 1451 269 Table 3 9443 1451 270 9443 1451 271 The fission cross section integral in the energy range 9443 1451 272 from 0.0021 eV to 3 eV. 9443 1451 273 9443 1451 274 ------------------------------------------------------------------9443 1451 275 Energy range This work ENDF/B-VI Wagemans et al. Weston and Todd9443 1451 276 (eV) (b.eV) (b.eV) (b.eV)(1) (b.eV)(8) 9443 1451 277 ------------------------------------------------------------------9443 1451 278 0.0021-0.020 31.06 30.61(-1.5%) 31.09(+0.1%) 9443 1451 279 0.0200-0.030 10.24 10.22(-0.2%) 10.24( 0.0%) 9443 1451 280 0.0300-0.100 49.02 50.02(+2.0%) 48.70(-0.6%) 9443 1451 281 0.1000-0.500 262.76 270.84(+3.1%) 264.58(+0.7%) 262.53(-0.1%) 9443 1451 282 0.5000-1.000 17.93 17.64(-1.6%) 17.60(-1.8%) 17.67(-1.4%) 9443 1451 283 1.0000-3.000 54.88 55.62(+1.3%) 54.40(-0.9%) 55.06(+0.3%) 9443 1451 284 ------------------------------------------------------------------9443 1451 285 0.0021-3.000 425.89 434.95(+2.1%) 426.61(+0.2%) 9443 1451 286 ------------------------------------------------------------------9443 1451 287 0.1000-3.000 335.57 344.10(+2.5%) 336.58(+0.3%) 335.26(-0.1%) 9443 1451 288 ------------------------------------------------------------------9443 1451 289 Weston and Todd experimental data were normalized to Wagemans et 9443 1451 290 al.(1) in the energy range from 0.1 eV to 12 eV (original EXFOR 9443 1451 291 data multiplied by 0.952). 9443 1451 292 9443 1451 293 9443 1451 294 Table 4 9443 1451 295 9443 1451 296 The capture cross section integral in the energy range from 9443 1451 297 from 0.0021 eV to3 eV. 9443 1451 298 9443 1451 299 -------------------------------------------------------------- 9443 1451 300 Energy range Present work ENDF/B-VI Weston and Todd(8) 9443 1451 301 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 302 -------------------------------------------------------------- 9443 1451 303 0.0021-0.020 12.25 12.28(+0.2%) 9443 1451 304 0.0200-0.030 3.67 3.68(+0.3%) 9443 1451 305 0.0300-0.100 15.28 15.39(+0.7%) 15.27(-0.1%) 9443 1451 306 0.1000-0.500 110.58 109.47(-1.0%) 110.49(-0.1%) 9443 1451 307 0.5000-1.000 5.90 5.87(-0.5%) 6.51 9443 1451 308 1.0000-3.000 7.30 7.14(-2.2%) 8.96 9443 1451 309 -------------------------------------------------------------- 9443 1451 310 0.0021-3.000 154.98 153.83(-0.7%) 9443 1451 311 -------------------------------------------------------------- 9443 1451 312 0.0300-3.000 139.06 137.87(-0.9%) 141.29(+1.6%) 9443 1451 313 -------------------------------------------------------------- 9443 1451 314 Weston and Todd experimental data were normalized to the cal- 9443 1451 315 culated average capture cross section over the resonance at 9443 1451 316 0.264 eV (original EXFOR data multiplied by 0.914); in the 9443 1451 317 energy range from 0.5 eV to 3 eV the experimental data are not 9443 1451 318 accurate due to large corrections for the impurities. 9443 1451 319 9443 1451 320 9443 1451 321 Table 5 9443 1451 322 9443 1451 323 The fission cross section integral in the energy range from 9443 1451 324 3 eV to 300 eV. 9443 1451 325 9443 1451 326 ------------------------------------------------------------------9443 1451 327 Energy range Present work ENDF/B-VI Weston and Todd(8) 9443 1451 328 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 329 ------------------------------------------------------------------9443 1451 330 3- 20 3038.63 3066.37(+0.9%) 3036.23(-0.1%) 9443 1451 331 20- 50 1683.69 1739.68(+3.3%) 1705.50(+1.3%) 9443 1451 332 50-100 1971.15 2030.10(+3.0%) 1931.50(-2.0%) 9443 1451 333 100-200 2554.85 2628.39(+2.9%) 2531.00(-0.9%) 9443 1451 334 200-300 2741.23 2820.75(+2.9%) 2747.00(+0.2%) 9443 1451 335 ------------------------------------------------------------------9443 1451 336 3-300 11989.55 12285.29(+2.5%) 11951.23(-0.3%) 9443 1451 337 ------------------------------------------------------------------9443 1451 338 Weston and Todd experimental data were normalized to Wagemans et 9443 1451 339 al.(1) in the energy range from 0.1 eV to 12 eV (original EXFOR 9443 1451 340 data multiplied by 0.952). 9443 1451 341 9443 1451 342 9443 1451 343 Table 6 9443 1451 344 9443 1451 345 The capture cross section integral in the energy range from 9443 1451 346 3 eV to 300 eV. 9443 1451 347 9443 1451 348 ------------------------------------------------------------------9443 1451 349 Energy range Present work ENDF/B-VI Weston and Todd(8) 9443 1451 350 (eV) (b.eV) (b.eV) (b.eV) 9443 1451 351 ------------------------------------------------------------------9443 1451 352 3- 20 1213.07 1138.52(-6.5%) 1192.90(-1.7%) 9443 1451 353 20- 50 330.34 307.48(-7.5%) 338.09(+2.3%) 9443 1451 354 50-100 605.40 585.88(-3.2%) 594.83(-1.8%) 9443 1451 355 100-200 609.83 581.77(-4.8%) 652.68(+7.0%) 9443 1451 356 200-300 684.97 661.12(-3.6%) 700.53(+2.3%) 9443 1451 357 ------------------------------------------------------------------9443 1451 358 3-300 3443.36 3274.77(-5.1%) 3479.04(+1.0%) 9443 1451 359 ------------------------------------------------------------------9443 1451 360 Weston and Todd experimental data normalized to the calculated 9443 1451 361 average capture cross section over the resonance at 0.265 eV 9443 1451 362 (original EXFOR data multiplied by 0.914). 9443 1451 363 9443 1451 364 $$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$$9443 1451 365 9443 1451 366 UNRESOLVED RESONANCE PARAMETERS START AT 300EV. 9443 1451 367 SAME AS VERSION V EXCEPT CAPTURE DOWN BY 4.8% AS 9443 1451 368 PER THE RECOMMENDATION OF H. DERRIEN AFTER THE STUDY9443 1451 369 OF THE WAGEMANS ET AL. DATA, REF 1. REVISION 1 HAD 9443 1451 370 CAPTURE DOWN BY 14% WHICH WAS DECIDED TO BE AN 9443 1451 371 OVERCORRECTION. FISSION IS UNCHANGED FROM VERSION 5 9443 1451 372 WHICH WAS BASED ON DATA OF SIMPSON, REF. 16, JAMES, 9443 1451 373 REF. 17, MIGNECO, REF. 10, BLONS, REF. 9, WESTON, 9443 1451 374 REF. 8, AND CARLSON, REF. 18. 9443 1451 375 MF=3 MT=1 TOTALS WERE REVISED FROM VERSION 5 TO REFLECT MORE 9443 1451 376 PHYSICAL SHAPE AS COMPARED TO PU239. 9443 1451 377 MF=3 MT=2 ADJUSTED TO BE CONSISTENT WITH TOTAL AND OTHER 9443 1451 378 PARTIAL CROSS SECTIONS. 9443 1451 379 MF=3 MT=18 ABOVE 40.2KEV SAME AS VERSION V AND BASED ON BEHRENS9443 1451 380 ,REF.15, KAPPELAR,REF.19, AND SZABO,REF.20, RATIOS 9443 1451 381 TO U235 WITH USE OF ENDF V EVALUATION OF U235. 9443 1451 382 MF=3 MT=102 RENORMALIZED DOWNWARD BY 4.8% FROM VERSION V. SEE 9443 1451 383 UNRESOLVED REGION ABOVE FOR EXPLAINATION. 9443 1451 384 MF=5 MT=16 REVISED BY R.J. HOWERTON FOR VERSION V. 9443 1451 385 MF=5 MT=17 REVISED BY R.J. HOWERTON FOR VERSION V. 9443 1451 386 MF=5 MT=18 FISSION NEUTRON ENERGY DISTRIBUTION GIVEN 9443 1451 387 AS SIMPLE FISSION SPECTRUM PLUS A 9443 1451 388 MAXWELLIAN (AWRE O-101/64) 9443 1451 389 MF=5 MT=91 REVISED BY R.J. HOWERTON FOR VERSION V. 9443 1451 390 MF=5,MT=455 DELAYED NEUTRON SECONDARY ENERGY DISTRIBUTION 9443 1451 391 SEE REF. 21. 9443 1451 392 MF=12 MT=18 USED DATA OF PEELE AND MAIENSCHEIN, REF 22, FOR 9443 1451 393 235-U THERMAL FISSION. 9443 1451 394 MF=12 MT=102 USED 238-U SPECTRUM ADJUSTED FOR MULTIPLICITY AND 9443 1451 395 ENERGY CONSERVATION. 9443 1451 396 MF=13 MT=3 CALCULATED BY R.J. HOWERTON 9443 1451 397 MF=15 MT=3 CALCULATED BY R.J. HOWERTON 9443 1451 398 MF=15 MT=18 CALCULATED BY R.J. HOWERTON. USED PEELE AND 9443 1451 399 MAIENSCHEIN DATA, REF 22, AND METHOD DESCRIBED 9443 1451 400 IN REF 23. 9443 1451 401 MF=15 MT=102 CALCULATED BY R.J. HOWERTON. 9443 1451 402 MF=33 MT=18,102 REPLACED BY L.WESTON DEC.1982 REF.24. 9443 1451 403 9443 1451 404 REFERENCES. 9443 1451 405 9443 1451 406 1. WAGEMANS,C. ET AL., Proc. Int. Conf. Nuc. Data for Sci. and 9443 1451 407 Tech., May 13-17, 1991, Julich, p. 35(1992). 9443 1451 408 2. DERRIEN,H. and de SAUSSURE,G.,Nuc.Sci.Eng.106,415(1990). 9443 1451 409 3. FREHAUT ET AL., CEA-R-4626, BRC(1974). 9443 1451 410 4. KAISER, R.E., CARPENTER, S.G.,(ANL-WEST) private comm.(1977).9443 1451 411 5. LARSON,N.M. and PEREY,F.G.,ORNL/TM-9719(1985). 9443 1451 412 6. WAGEMANS,C.,SCHILLEBEECKX,P.,DERUYTTER,A. and 9443 1451 413 BARTHELEMY,R.,Proc.Int.Conf.,PHYSOR 90,Marseille,France, 9443 1451 414 Vol.1,III-9(1990). 9443 1451 415 7. WAGEMANS,C. and DERUYTTER,A.,Nucl.Sci.Eng.60,44(1976). 9443 1451 416 8. WESTON,L.W. and TODD,J.H.,Nucl.Sci.Eng.65,454(1978). 9443 1451 417 9. BLONS,J.,Nucl.Sci.Eng.51,130(1973). 9443 1451 418 10. 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TO B.A.MAGURNO NOV.12,1982 9443 1451 442 * * * * * *9443 1451 443 9443 1451 444 1 451 516 19443 1451 445 1 452 5 09443 1451 446 1 455 7 09443 1451 447 1 456 5 09443 1451 448 1 458 5 09443 1451 449 2 151 409 19443 1451 450 3 1 39 09443 1451 451 3 2 39 09443 1451 452 3 4 37 09443 1451 453 3 16 17 09443 1451 454 3 17 8 09443 1451 455 3 18 39 09443 1451 456 3 51 21 09443 1451 457 3 52 18 09443 1451 458 3 53 17 09443 1451 459 3 54 16 09443 1451 460 3 55 16 09443 1451 461 3 56 15 09443 1451 462 3 57 15 09443 1451 463 3 58 14 09443 1451 464 3 59 14 09443 1451 465 3 60 13 09443 1451 466 3 61 12 09443 1451 467 3 62 11 09443 1451 468 3 63 11 09443 1451 469 3 64 10 09443 1451 470 3 65 10 09443 1451 471 3 91 26 09443 1451 472 3 102 39 19443 1451 473 4 2 133 09443 1451 474 4 16 10 09443 1451 475 4 17 10 09443 1451 476 4 18 10 09443 1451 477 4 51 10 09443 1451 478 4 52 10 09443 1451 479 4 53 10 09443 1451 480 4 54 10 09443 1451 481 4 55 10 09443 1451 482 4 56 10 09443 1451 483 4 57 10 09443 1451 484 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