29-Cu-nat from T508 508 0 0 0 2.90000+ 4 6.35460+ 1 1 0 0 11329 1451 1 0.00000+ 0 0.00000+ 0 0 0 0 01329 1451 2 0.00000+ 0 0.00000+ 0 0 0 282 581329 1451 3 29-cu- ornl,sai eval-dec73 fu,drake,fricke 1329 1451 4 dna-3356f(1974) dist-jan79 rev1-mar78 790109 1329 1451 5 dna-3356f discribes endf/b-iv. revisions for endf/b-v and 1329 1451 6 dna-4529 mod 2 are summarized below and will be published. 1329 1451 7 ***** summary for endf/b-v and dna-4529 mod 2 (c. y. fu, 1978) ***1329 1451 8 3-1 total cross sections from 0.2 to 2.0 mev were replaced by the1329 1451 9 high-resolution cross sections measured by perey(1). these data 1329 1451 10 seemed to be of the highest quality available. 1329 1451 11 3-2 elastic scattering cross sections were obtained by 1329 1451 12 subtracting the nonelastic from the total. 1329 1451 13 3-3 nonelastic cross sections were changed due to revisions 1329 1451 14 in (n,p), (n,a), (n,np), and (n,na) cross sections. 1329 1451 15 3-22 (n,na) cross sections were changed due to revisions in both 1329 1451 16 isotopes. cu-63(n,na) cross sections were based on our calculated1329 1451 17 curve(2) normalized at 14.8 mev to the helium production cross 1329 1451 18 sections for cu-63 measured by grimes and haight(3) with fixed 1329 1451 19 cu-63(n,a) cross sections (see 3-107). cu-65(n,na) cross sections1329 1451 20 were based on the data of santry and butler(4). 1329 1451 21 3-28 (n,np) cross sections were modified due to revisions in both1329 1451 22 isotopes. cu-63(n,np) cross sections were based on our analysis(5)1329 1451 23 of the proton spectrum from 14.8-mev neutrons incident on cu-63 1329 1451 24 measured by grimes and haight(3). cu-65(n,np) cross sections 1329 1451 25 below 12 mev were based on the calculation of mann(6); from 12 to 1329 1451 26 20 mev mann s calculation was slightly modified to reproduce the 1329 1451 27 14.8-mev hydrogen production cross section of cu-65 measured by 1329 1451 28 grimes and haight(3) with fixed cu-65(n,p) cross sections(see 1329 1451 29 3-103). 1329 1451 30 3-102 (n,g) cross sections were thinned to 1%, reducing the 1329 1451 31 number of energy entries from 408 to 48. this automatically 1329 1451 32 shortened files 3-1, 3-2 and 3-3. 1329 1451 33 3-103 (n,p) cross sections were changed due to revision of 1329 1451 34 cu-63(n,p) cross sections, which were based on model analysis(5) 1329 1451 35 of the proton spectrum from 14.8-mev neutrons incident on cu-63 1329 1451 36 measured by grimes and haight(3). cu-65(n,p) cross sections were 1329 1451 37 taken from the evaluation by drake and fricke(7) which has 1329 1451 38 adequate data basis. 1329 1451 39 3-107 cu-63(n,a) cross sections were taken from endf/b-iv 1329 1451 40 dosimetry file mat 6411(8). cu-65 (n,a) cross sections below 1329 1451 41 10 mev were taken from the calculation by mann(6). from 10 mev 1329 1451 42 to 20 mev mann s calculation was altered to reproduce the 14.8-mev1329 1451 43 helium production cross section measured by grimes and haight(3) 1329 1451 44 with fixed cu-65(n,na) cross sections (see 3-22). 3-107 and 1329 1451 45 3-22 together yield a helium production cross section of 51 mb 1329 1451 46 at 14.8 mev for natural copper, in good agreement with a measured 1329 1451 47 value of 52+-4 mb by farrar et al.(9). 1329 1451 48 12-102 capture gamma-ray multiplicities from 0.2 to 1.25 mev were 1329 1451 49 revised according to the measurement by chapman(10) and 3-102. 1329 1451 50 15-102 two energy distributions of the secondary gamma rays from 1329 1451 51 capture for incident neutron energies from 0.2 to 1.25 mev were 1329 1451 52 added(10). in the previous evaluation, thermal capture gamma rays1329 1451 53 were used in the above energy range. 1329 1451 54 1. f. g. perey, oak ridge national laboratory, private 1329 1451 55 communication(1977). 1329 1451 56 2. c. y. fu and f. g. perey, j. nucl. mater. 61, 153(1976). 1329 1451 57 3. s. m. grimes and r. c. haight, lawrence livermore laboratory, 1329 1451 58 private communication(1977) 1329 1451 59 4. d. c. santry and j. p. butler,can. j. phys. 44,1153(1965). 1329 1451 60 5. c. y. fu, ornl-tm(to be published). 1329 1451 61 6. f. m. mann, hanford engineering development laboratory, 1329 1451 62 private communition(1977). 1329 1451 63 7. m. k. drake and m. p. fricke, science applications inc., 1329 1451 64 dna-3356f(1974). 1329 1451 65 8. h. alter, in endf/b-iv dosimetry file, ed. b. a. magurno, 1329 1451 66 bnl-ncs-50446, endf-216(1975). 1329 1451 67 9. h. farrar et al., atomics international, private communication1329 1451 68 (1977). 1329 1451 69 10. g. t. chapman, oak ridge national laboratory, ornl-tm-5215 1329 1451 70 (1976). 1329 1451 71 **summary for dna 4529 mod 1 (m. k. drake and m. p. fricke,1974)**1329 1451 72 *** resonance parameters (file 2) *** 1329 1451 73 resonance parameters and file-3 cross sections below 30 kev 1329 1451 74 were taken from endf/b-iii (1) which was based on bnl-325(2). 1329 1451 75 total cross section (mt=1) * * * * * * * * * * * * * * * * * 1329 1451 76 between 30 kev and 100 kev, the data measured by garg, et.al. 1329 1451 77 (3) were used. in this energy range there was considerable 1329 1451 78 structure in the experimental data, but it was not measured 1329 1451 79 well enough to obtain resolved resonance parameters. in the en. 1329 1451 80 region from 100 kev to 1.5 mev, the anl results obtained by 1329 1451 81 meadows and whalen (4) were used. in the upper portion of this 1329 1451 82 energy range (1.2 to 1.5 mev) the experimental data were averaged1329 1451 83 over 200 kev energy bands since the variations in the experiment-1329 1451 84 tal data appeared to be more statistical than structure in c/s. 1329 1451 85 very poor quality data were available for the region from 1.5 1329 1451 86 to 2.3 mev (5,6). a smooth curve was drawn for the total cross 1329 1451 87 section. the curve did not go through the average of the data, 1329 1451 88 rather the curve was drawn to fit the better data below 1.5 mev 1329 1451 89 and above 2.3 mev. between 2.3 and 12 mev, a smooth curve was 1329 1451 90 drawn through the foster and glasgow (7) data. an average of the 1329 1451 91 data measured by foster and glasgow (7), albergotti and ferguson 1329 1451 92 (8), and robinson, et.al.(9) were used for neutron energies 1329 1451 93 between 12 and 15 mev. above 15 mev a smooth and slowly decres- 1329 1451 94 ing curve was drawn through the available data (10,11,12,13). 1329 1451 95 * *elastic scattering cross section (mt=2) * * * * * * * * * * * 1329 1451 96 by subtracting the non-elastic cross section from the evaluated 1329 1451 97 total cross section. the resulting cross section was compared to 1329 1451 98 the available experimental data for elastic scattering. in the 1329 1451 99 energy region from 0.3 to 4.0 mev, the evaluated cross section 1329 1451 100 agreed very well with the available measurements (14,15,16,17). 1329 1451 101 between 4 and 8 mev, the evaluated curve was slighly higher 1329 1451 102 than the measured data of holmqvist (17). 1329 1451 103 * *non-elastic cross section (mt=3) * * * * * * * * * * * * * * 1329 1451 104 below 600 kev, the non-elastic cross section was the same as the 1329 1451 105 radiative capture cross section. between 600 kev and 5 mev, the 1329 1451 106 non-elastic cross sections for the isotopes were obtained by 1329 1451 107 summing the components. above 5 mev, the non-elastic cross 1329 1451 108 sections for the isotopes were taken to be the same as the 1329 1451 109 element which was evaluated by drawing a smooth curve through 1329 1451 110 the existing experimental data (18,19,20,21,22,23,24,25,26,27). 1329 1451 111 in the energy range from 6 to 9 mev, there was a discrepancy 1329 1451 112 between the available experimental data for elastic scattering 1329 1451 113 (17) and non-elastic cross section (18,20). the evaluated cross 1329 1451 114 section for both the elastic and non-elastic cross sections were 1329 1451 115 slighly higher than the experimental data. this was done to 1329 1451 116 preserve the total c/s which was measured more accurately. 1329 1451 117 * *(n,2n) cross section (mt=16) * * * * * * * * * * * * * * * * 1329 1451 118 many sets of experimental data were available for cu-63. some 1329 1451 119 were absolute and others were relative. the relative measurements1329 1451 120 (28,29,30,31,32) were re-normalized to 0.568 barns at 14.7 mev, 1329 1451 121 consistent with the cu-65 (n,2n) cross section at this energy 1329 1451 122 the absolute values (33,34,35,36) along with the results from 1329 1451 123 14 mev measurements and the re-normalized cross section values 1329 1451 124 were used to obtain the recommended cross section. 1329 1451 125 the cu-65 (n,2n) cross section was taken from the endf/b 1329 1451 126 dosimetry library. this evaluation was based on measurements by 1329 1451 127 santry and butler (37), prestwood and bayhurst (38), paulsen and 1329 1451 128 liskien (39), rayburn (31), and bormann and lammers (36). 1329 1451 129 * *(n,p) and (n,n-p) cross sections (mt=28,103) * * * * * * * * 1329 1451 130 very little experimental data were available for cu-63 (n,p) or 1329 1451 131 cu-63 (n,n-p). these cross sections were obtained from statistic-1329 1451 132 al model calculations. the calculated results were normalized at 1329 1451 133 14.5 mev to the sparce experimental data (40,41,42,43) 1329 1451 134 the (n,p) cross section for cu-65 has been measured from 1329 1451 135 threshold (about 3 mev) to 20 mev. the data of santry and butler 1329 1451 136 (37) were used for the complete energy range. the magnitude of 1329 1451 137 the cross section near 14 mev was well established by several 1329 1451 138 other measurements. few and widely disagreeing values have been 1329 1451 139 measured for the (n,n-p) c/s. the same procedure for cu-63 1329 1451 140 (n,n-p) was used for cu-65 (n,n-p) c/s. 1329 1451 141 * *(n,alpha) and (n,n-alpha) cross sections (mt=22,107) * * * * 1329 1451 142 the cu-63(n,a) c/s was taken from the endf/b dosimetry 1329 1451 143 file. this evaluation was based on the data of paulsen and 1329 1451 144 liskien (44). the (n,n-alpha) cross section for cu-63 was based 1329 1451 145 on a statistical model calculation which was normalized to an 1329 1451 146 experimental value at 14.8 measured by irfan and jack (45). 1329 1451 147 the (n,alpha) cross section for cu-65 was based on a 1329 1451 148 statistical model calculation and the calculated curve was 1329 1451 149 normalized to the available experimental data(46,47,48) at 1329 1451 150 14 mev. the (n,n-alpha) cross section was based on the experi- 1329 1451 151 mental data of santry and butler (37), bramlitt and fink (46), 1329 1451 152 and kantele and gardner (49). 1329 1451 153 * *radiative capture cross section (mt=102) * * * * * * * * * * 1329 1451 154 above 30 kev, the radiative capture cross section was obtained1329 1451 155 by evaluating this cross section for the isotopes. between 30 kev1329 1451 156 and 3 mev, the cu-63 (n,g) cross section was based on the experi-1329 1451 157 mental data of dovbenko, et.al. (50) and zaikin, et.al.(51). 1329 1451 158 the recommended curve was drawn slighly higher than the dovbenko 1329 1451 159 data and lower than the zaikin data. at 14 mev, the curve was 1329 1451 160 drawn through perkin (52) and a recent columbia value (53). 1329 1451 161 the cu-65 (n,g) cross section curve was drawn through 46 mb 1329 1451 162 at 25 kev, which was an average of several mono-energetic measur-1329 1451 163 ements between 20 and 25 kev. above 30 kev, the recommended curve 1329 1451 164 was drawn on the low side of values measured by tolstikov (54) 1329 1451 165 and stavisskii and tolstikov (55). between 600 kev and 3 mev, 1329 1451 166 the data measured by zaikin, et.al, were used. 1329 1451 167 * *inelastic scattering cross sections (mt=4,51,52,..,91) * * * 1329 1451 168 the inelastic scattering cross section was made up of 11 1329 1451 169 discrete levels and a continuum. several sets of inelastic 1329 1451 170 scattering and gamma ray production cross section measurements 1329 1451 171 were used to obtained the level excitation cross sections for 1329 1451 172 neutron energies up to 1.5 mev (14,56,57,58,59) for the 0.67 1329 1451 173 and 0.912 mev levels in cu-63 and the 0.77 and 1.115 mev levels 1329 1451 174 in cu-65. from 5.5 to 8 mev, the data of kinney(59a) were used. 1329 1451 175 extrapolation to other energies was based on helene and dwuck 1329 1451 176 calculations. 1329 1451 177 * * * * * file 4 (angular distributions for secondary neutrons) 1329 1451 178 * *elastic scattering (mt=2) * * * * * * * * * * * * * * * * * 1329 1451 179 isotropic below 100 kev. between 100 kev and 600 kev the 1329 1451 180 data of lane, et.al (60) were used. between 600 kev and 1.2 mev,1329 1451 181 the data measured by cox (61) were used and between 1.5 and 8 mev1329 1451 182 the measurement made by holmqvist (17) was used. near 14 mev the 1329 1451 183 results from several measuremnts were used (62,63,64). from 8 1329 1451 184 to 14 mev and above 15 mev, the angular distributions were 1329 1451 185 calculated using the helene and dwuck codes. 1329 1451 186 * *non-elastic reaction (mt=51,52,..,91,22,28,16) * * * * * * * 1329 1451 187 angular distributions for neutrons from inelastic level 1329 1451 188 reactions were obtained from the helene code (compound nucleus 1329 1451 189 part) and the dwuck code (direct interaction part). calculations 1329 1451 190 were made for the first 3 levels in each isotpe. there was 1329 1451 191 reasonably good agreement between the calculated distributions 1329 1451 192 for the 0.77 and 1.115 mev levels at 2.33 mev and a measurement 1329 1451 193 by rogers et.al.(65). all other levels , the continuum, and all 1329 1451 194 other neutron producing reactions were assumed to have isotropic 1329 1451 195 distributions in the c.m. system. 1329 1451 196 * * * * * file 5 (energy distributions for secondary neutrons) 1329 1451 197 the energy distributions for inelastic scattering continuum 1329 1451 198 (mt=91) and (n,2n) (mt=16) were based on the statistical model. 1329 1451 199 an effective nuclear temperaure of 1.02 mev at 14.1 mev was 1329 1451 200 used. the effective nuclear temperature of the second neutron for1329 1451 201 the (n,2n) reaction was 0.4 mev at 14 mev. 1329 1451 202 * * * * * file 12 (multiplicities for radiative capture) * * * * 1329 1451 203 the multiplicities for radiative capture gamma rays was taken 1329 1451 204 from a thermal neutron measurement made by orphan, et.al (66). 1329 1451 205 * * * * file 13 (n,n-g) and (n,2n-g) gamma ray production 1329 1451 206 cross sections * * * * * * * * * * * * * * * * * * * * 1329 1451 207 spec10 calculations fitting data of jonsson(67) and dickens(68)1329 1451 208 * * * * * file 15 (energy distributions for secondary gamma rays)1329 1451 209 orphan et al.(66) for capture gamma rays. dickens et al.(68) 1329 1451 210 for gamma rays from all reactions above 1.25 mev. 1329 1451 211 (1) j.m.otter,et.al., report ai-aec-1271 (1968) 1329 1451 212 (2) m.d.goldberg, et.al., bnl-325, 2nd ed., suppl. 2, vol iia 1329 1451 213 (1966) 1329 1451 214 (3) j.b.garg, j.rainwater, and w.w.havens,jr., report 1329 1451 215 eandc(us)- 54 l (1964) 1329 1451 216 (4) j.w.meadows and j.f. whalen (anl) pri.comm. (1972) 1329 1451 217 (5) m.n.nikolayev. et.al., phys of fast and intermediate 1329 1451 218 reactors, vol.i, (1961) 1329 1451 219 (6) d.w.miller, et.al., phys.rev. 88, 1042 (1952) 1329 1451 220 (7) d.g.foster,jr. and d.w. glasgow, phys.rev. 3,c576 (1971) 1329 1451 221 (8) j.c.albergotti and j.m.ferguson, nucl.phys. 82,652 (1966) 1329 1451 222 (9) w.k.robinson, et.al., american j.phys. 37,482 (1969) 1329 1451 223 (10) p.h.bowen, et.al., nucl.phys. 22,640 (1960) 1329 1451 224 (11) j.m.peterson, et.al., phys.rev. 120,521 (1960) 1329 1451 225 (12) r.b.day and r.l.henkel, phys.rev. 92,358 (1958) 1329 1451 226 (13) m.mazari, et.al., phys. rev. 100,972 (1955) 1329 1451 227 (14) a.b.smith, et.al., phys. rev. 135,76 (1964) 1329 1451 228 (15) i.a.korzh, et.al., at. en. 16,260 (1964) 1329 1451 229 (16) l.ya.kasakova, et.al., conf. on nuclear structure study 1329 1451 230 with neutrons, p 200, antwerp (1965) 1329 1451 231 (17) b.holmqvist, arkiv fysik 38,403 (1968) 1329 1451 232 (18) j.r.beyster, et.al., phys.rev. 104,1319 (1956) 1329 1451 233 (19) h.l.taylor, et.al., phys.rev. 100,174 (1955) 1329 1451 234 (20) w.p.ball, et.al., phys.rev. 110,1392 (1958) 1329 1451 235 (21) t.w.bonner and j.c. slattery, phys.rev. 113,1088 (1959) 1329 1451 236 (22) g.m.haas and p.l.okhuysen, phys.rev. 132,1211 (1963) 1329 1451 237 (23) d.d.phillips, et.al., phys.rev. 88,600 (1952) 1329 1451 238 (24) m.h.mac gregor, et.al., phys.rev. 108,726 (1957) 1329 1451 239 (25) d.didier, et.al., report eandc(e) - 49 l (1963) 1329 1451 240 (26) a.chatterjee and a.m.ghose, phys.rev. 161,1181 (1967) 1329 1451 241 (27) yu.g.degtyarev and v.g.nadtochii, at.en. 11, 397 (1961) 1329 1451 242 (28) d.r.kohler and w.l.alford, report aomc-rr-62-1 (1969) 1329 1451 243 (29) a.v.cohen and p.h.white, nucl.phys. 1, 73 (1956) 1329 1451 244 (30) j.c.csikai and g.peto, actaphys.acad.sci.hungaricae 1329 1451 245 23, 87 (1967) 1329 1451 246 (31) l.a.rayburn, phys.rev. 130, 731 (1963) 1329 1451 247 (32) r.n.glover and e.weigold, nucl.phys. 29, 309 (1962) 1329 1451 248 (33) w.e.thomson and j.m.ferguson, phys.rev. 118, 228 (1960) 1329 1451 249 (34) m.bormann, et.al., z.physik 166, 477 (1962) 1329 1451 250 (35) h.liskien and a.paulsen, j.nucl.energy a/b 19, 73 (1965) 1329 1451 251 (36) m.bormann and b.lammers, nucl.phys. a130, 195 (1969) 1329 1451 252 (37) d.c.santry and j.p.butler, can.j.phys. 44, 1183 (1966) 1329 1451 253 (38) r.j.prestwood and b.p.bayhurst, phys.rev. 121, 1438 (1961) 1329 1451 254 (39) a.paulsen and h.liskien, nukleonik 7, 117 (1965) 1329 1451 255 (40) d.l.allan, nucl.phys. 24,274 (1961) 1329 1451 256 (41) r.s.storey, et.al., proc.phys.soc. 75,526 (1960) 1329 1451 257 (42) l.colli, et.al., nuovo cimento 13, 730 (1959) 1329 1451 258 (43) d.l.allan, proc.phys.soc. 70, 195 (1957) 1329 1451 259 (44) a.paulsen, nukleonik 10, 91 (1967) 1329 1451 260 (45) m.irfan and w.jack, proc.phys.soc. 81, 808 (1963) 1329 1451 261 (46) e.t.bramlitt and r.w.fink, phys.rev. 131, 2649 (1963) 1329 1451 262 (47) i.l.priess and r.w.fink, nucl.phys. 15, 626 (1960) 1329 1451 263 (48) d.l.claytor, dissertation abstr. 30b, 2850 (1969) 1329 1451 264 (49) j.kantele and d.g.gardner, nucl.phys. 35, 353 (1962) 1329 1451 265 (50) a.g.dovbenko, et.al., report indc-260 e, p 11 (1969) 1329 1451 266 (51) g.g.zaikin, et.al., at.en. 25,526 (1968) 1329 1451 267 (52) j.l.perkin, proc.phys.soc. 72, 505 (1958) 1329 1451 268 (53) m.stamatelatos, pri.comm. (1972) 1329 1451 269 (54) v.a.tolstikov, et.al., at.en. 17, 505 (1964) 1329 1451 270 (55) yu.ya.stavisskii and v.a.tolstikov, at.en. 10, 508 (1961) 1329 1451 271 (56) n.p.glazkov, at.en. 15,416 (1963) 1329 1451 272 (57) a.b.tucker, et.al., phys.rev. 137, 1181 (1965) 1329 1451 273 (58) b.holmqvist and t.wiedling, arkiv fysik 35, 71 (1967) 1329 1451 274 (59) k.nishimura, et.al., nucl.phys. 70, 421 (1965) 1329 1451 275 (59a) w. e. kinney, ornl-4908(1974). 1329 1451 276 (60) r.o.lane, et.al., ann.phys. 12, 135 (1961) 1329 1451 277 (61) s.a.cox, bull.am.phys.soc 8, 478 (1963) 1329 1451 278 (62) j.h.coon, et.al., phys.rev. 111, 250 (1958) 1329 1451 279 (63) s.berko, et.al., nucl.phys. 6, 210 (1958) 1329 1451 280 (64) b.ya.guzhovski, at.en. 11, 395 (1961) 1329 1451 281 (65) w.l.rogers, et.al., report coo-1573-33 (1967) 1329 1451 282 (66) v.j.orphan, et.al., report ga-10248 (1970) 1329 1451 283 (67) b.jonsson, et.al., arkiv fysik 39, 295 (1969) 1329 1451 284 (68) j. k. dickens et al., ornl-4840(1973). 1329 1451 285 1 451 343 11329 1451 286 2 151 57 01329 1451 287 3 1 496 11329 1451 288 3 2 412 11329 1451 289 3 3 102 11329 1451 290 3 4 68 01329 1451 291 3 16 10 01329 1451 292 3 17 4 01329 1451 293 3 22 11 11329 1451 294 3 28 12 11329 1451 295 3 51 54 01329 1451 296 3 52 47 01329 1451 297 3 53 40 01329 1451 298 3 54 34 01329 1451 299 3 55 29 01329 1451 300 3 56 27 01329 1451 301 3 57 27 01329 1451 302 3 58 25 01329 1451 303 3 59 25 01329 1451 304 3 60 22 01329 1451 305 3 61 22 01329 1451 306 3 91 22 01329 1451 307 3 102 19 11329 1451 308 3 103 13 11329 1451 309 3 104 11 01329 1451 310 3 106 9 01329 1451 311 3 107 24 11329 1451 312 3 251 18 01329 1451 313 3 252 18 01329 1451 314 3 253 18 01329 1451 315 4 2 188 01329 1451 316 4 16 10 01329 1451 317 4 17 10 01329 1451 318 4 22 10 01329 1451 319 4 28 10 01329 1451 320 4 51 91 01329 1451 321 4 52 91 01329 1451 322 4 53 91 01329 1451 323 4 54 91 01329 1451 324 4 55 85 01329 1451 325 4 56 10 01329 1451 326 4 57 85 01329 1451 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