Be-9 404 0 0 0 4.00900+ 3 8.93480+ 0 0 0 6 411289 1451 1 0.00000+ 0 0.00000+ 0 0 0 281 01289 1451 2 4-be- 9 lll eval-dec71 howerton, perkins 1289 1451 3 dist-may74 rev-nov74 1289 1451 4 1289 1451 5 ********************* dna 4154 mod 2 ********************* 1289 1451 6 1289 1451 7 the (n,2n) reaction was described using format modification 73-4 1289 1451 8 which allows the representation of individual neutrons from 1289 1451 9 sequential (n,2n) reactions. this was done utilizing mt=6-9 and 1289 1451 10 46-49 in files 3 and 4, and mt=46-49 in file 5. 1289 1451 11 mt = 105 now includes (n,t0) in addition to (n,t1) data. 1289 1451 12 the (n,t) reaction was split into (n,t0) and (n,t1) components 1289 1451 13 using mt = 740 and 741. 1289 1451 14 1289 1451 15 ************************************************************** 1289 1451 16 1289 1451 17 1289 1451 18 ********************** dna 4154 mod 1 ****************** 1289 1451 19 1289 1451 20 1. the energy range was extended down to 1.0e-05 ev. 1289 1451 21 1289 1451 22 2. gamma ray production for (n,g) and (n,t) are now 1289 1451 23 represented as mt=102 and mt=105, respectivly, 1289 1451 24 in files 12 and 15. the photon spectrum from 1289 1451 25 capture was assumed independent of incident neutron 1289 1451 26 energy with the multiplicity varied with incident 1289 1451 27 neutron energy to conserve energy. 1289 1451 28 1289 1451 29 ********************************************************** 1289 1451 30 1289 1451 31 be-9 evaluated neutron cross sections 1289 1451 32 for endf/b iv and dna library 1289 1451 33 evaluated by r.j.howerton and s.t.perkins 1289 1451 34 lawrence livermore laboratory, livermore, ca. 1289 1451 35 september, 1973 1289 1451 36 1289 1451 37 general comments 1289 1451 38 the neutron energy range covered extends from .00001 ev to 1289 1451 39 20 mev. in addition to elastic scattering which of course is 1289 1451 40 everywhere energetically possible, the following reactions have 1289 1451 41 thresholds (ucrl 50400, vol. 9) at energies less than 20 mev 1289 1451 42 reaction threshold (mev) 1289 1451 43 n,2n 1.85 1289 1451 44 n,p 14.26 1289 1451 45 n,np 18.76 1289 1451 46 n,d 16.29 1289 1451 47 n,nd 18.55 1289 1451 48 n,t 11.60 1289 1451 49 n,nt 19.65 1289 1451 50 n,alpha 0.67 1289 1451 51 n,n alpha 2.74 1289 1451 52 n,gamma exoergic 1289 1451 53 for the (n,np), (n,nd), and (n,nt) reactions, there are 1289 1451 54 no measurements and since the thresholds are sufficiently 1289 1451 55 high, these cross sections will be considered negligible. the 1289 1451 56 (n,n alpha) reaction is in reality a decay mode for the (n,2n) 1289 1451 57 reaction since he-5 is unstable, decaying immediately to a 1289 1451 58 neutron and an alpha particle. additionally, the inelastic 1289 1451 59 scattering reaction is also a decay mode for the (n,2n) reaction 1289 1451 60 since the be-9* recoil nucleus always decays to the final end 1289 1451 61 products of a neutron and two alpha particles. the way in which 1289 1451 62 the cross sections are selected for elastic scattering, (n,2n), 1289 1451 63 (n,p), (n,d), (n,t), (n, alpha), (n, gamma), as well as the 1289 1451 64 (n,x gamma) reaction is discussed below. 1289 1451 65 1289 1451 66 elastic scattering cross section 1289 1451 67 in keeping with the principle established for the entire 1289 1451 68 lll evaluated cross section library, the free atom cross section 1289 1451 69 is used for all energies below the usual upper limit of the 1289 1451 70 molecular binding energy (about 10 ev). this is effectively only 1289 1451 71 the nuclear part of the cross section of a stationary target at 1289 1451 72 zero degrees kelvin. it is stroncly emphasized that the numbers 1289 1451 73 are meaningless in the absence of a proper thermal treatment by 1289 1451 74 either the processing code or the neutronics code which uses 1289 1451 75 these numbers. they are likewise meaningless if the materials for1289 1451 76 which they are to be used are bound in molecules unless molecular1289 1451 77 binding is taken into account. 1289 1451 78 the scattering cross section was taken equal to 6 barns 1289 1451 79 from 0.00001 ev to 0.01 mev. from .01 mev to the 1289 1451 80 (n,alpha) threshold at 0.67 mev, the scattering cross section is 1289 1451 81 equal to the total cross section since the (n,gamma) cross 1289 1451 82 section is negligible. the cross section was 1289 1451 83 based on data of refs. 63, 92, 720, 772 and 1002. 1289 1451 84 above the (n,alpha) threshold, the scattering cross section 1289 1451 85 was taken as the difference between the total and the nonelastic,1289 1451 86 with the nonelastic being equal to the sum of its parts. up to 21289 1451 87 mev, the total cross section was based on the previously 1289 1451 88 mentioned data, as well as that from refs. 72, 336 and 1642. 1289 1451 89 above this energy, we relied on the results of ref. 3088 1289 1451 90 over the 2.7 mev resonance, and ref. 750 up to 15 mev. the 1289 1451 91 extension to 20 mev utilized data from refs. 107, 673 and 682. 1289 1451 92 1289 1451 93 elastic scattering angular distributions, 1289 1451 94 (normalized probabilities) 1289 1451 95 up to 7 mev, there are experimental differential scattering 1289 1451 96 data in refs. 121, 151, 231, 296, 500, 571, 945, 1643, 1645, 16461289 1451 97 and 1647. these results were used to determine the normalized 1289 1451 98 probabilities. in be below the (n,2n) threshold, the total 1289 1451 99 scattering data is equivalent to that for elastic scattering, 1289 1451 100 since there is no inelastic scattering. the change in 1289 1451 101 shape of the angular distribution going through the scattering 1289 1451 102 resonances was taken into account. at 14 mev, the probabilities 1289 1451 103 were based on the results of ref. 402, 2585 and 3106. a smooth 1289 1451 104 extrapolation was made to 20 mev. 1289 1451 105 1289 1451 106 (n,2n) cross section 1289 1451 107 the total (n,2n) cross section is based on the (n,2n) 1289 1451 108 cross sections, and nonelastic minus absorption cross sections 1289 1451 109 referenced in perkins (an-1443, 1965), as well as the new n,2n 1289 1451 110 data given in ref. 763 and 3320 and the new nonelastic results of1289 1451 111 ref. 2595 and 3321. the 20 mev point was based on interpolating 1289 1451 112 nonelastic cross sections between the 14 mev value and the value 1289 1451 113 at 25.5 mev quoted in ref. 356. the total (n,2n) cross section 1289 1451 114 was then subdivided into 4 partial reactions which were described1289 1451 115 by time-sequential decays, be-9(n,n1)be-9*(n2)be-8*. 1289 1451 116 levels excited were at 1.68, 2.43, 6.76, and 11.28 mev in be-9*, 1289 1451 117 and 0., 2.94, and 11.4 mev in be-8*. branching ratios were taken 1289 1451 118 from perkins (an-1443,1965) with, however, the be-9* (9.1) 1289 1451 119 transition being replaced by be-9* (11.28). 1289 1451 120 1289 1451 121 (n,2n) first neutron 1289 1451 122 for each of the partial (n,2n) reactions, the first 1289 1451 123 neutron is described as an inelastic scattering event. the 1289 1451 124 center of mass angular distribution of the (n,nprime) 1289 1451 125 neutron from be-9*(2.43) was described by a p6 legendre 1289 1451 126 expansion - data taken from perkins (an-1443,1965) and smoothly 1289 1451 127 extrapolated to 20 mev. all other reactions were assumed 1289 1451 128 isotropic in their center of mass systems. 1289 1451 129 1289 1451 130 (n,2n) second neutron 1289 1451 131 the description of the second neutron from each 1289 1451 132 partial reaction neglects the energy-angle correction. this 1289 1451 133 is a valid approximation for this reaction, as has been 1289 1451 134 discussed previously (nse 31,156(1968)). the energy spectra 1289 1451 135 are given by pi0(e to e2) with the lab system angular 1289 1451 136 distributions described by a p9 expansion of the transference 1289 1451 137 function. except for be-9* (2.43) and be-8*(0.), all levels were 1289 1451 138 described by single level dispersion theory (widths taken 1289 1451 139 from lap-117,1973 and lap-118,1973). all moments of the 1289 1451 140 transference function were then integrated over the level 1289 1451 141 distributions (equations in an-1443,1965). the integration 1289 1451 142 scheme used bins of equal probability which has introduced 1289 1451 143 some discontinuties into the output spectra, particularly 1289 1451 144 at low incident neutron energies. 1289 1451 145 1289 1451 146 (n,p) cross section 1289 1451 147 this cross section was estimated from the known threshold 1289 1451 148 value and the single measurement at 15.5 mev given in ref. 913. 1289 1451 149 1289 1451 150 (n,d) cross section 1289 1451 151 this cross section is based in its entirety on the data 1289 1451 152 between 16.5 and 18.8 mev reported in ref. 3101. 1289 1451 153 1289 1451 154 (n,t) cross section 1289 1451 155 the cross section for the (n,t) reaction is based on a 1289 1451 156 (n,t0) and a(n,t1) component, which proceed through the 0. and 1289 1451 157 the 0.477 mev levels in li-7* respectively. the total (n,t) 1289 1451 158 cross section near 14 mev was determined from ref. 496 and 650. 1289 1451 159 the results of ref. 494 were neglected due to the large 1289 1451 160 uncertanties. 1289 1451 161 the (n,t1) cross section was based on the work in ref. 605 1289 1451 162 from 13.6 - 14.7 mev. above this energy, there is a resonance 1289 1451 163 structure seen in the total cross section reported in ref. 107 1289 1451 164 and 682. this was assumed to be due to the (n,t1) reaction and is1289 1451 165 not in conflict with the rapid increase in the cross section 1289 1451 166 above 14.5 mev seen by ref. 605. 1289 1451 167 1289 1451 168 (n,alpha) cross section 1289 1451 169 the cross section was based on the measurements reported 1289 1451 170 in ref. 160, 494 and 733 up to neutron energies of 8.6 mev. it 1289 1451 171 was then tied into the three values given at 14 mev, refs. 86, 1289 1451 172 650 and 2367, and then smoothly extrapolated to 20. mev. note 1289 1451 173 that the measured cross section is to he-6(0. mev) which beta 1289 1451 174 decays to li-6, higher states in he-6 decay to alpha + 2n. 1289 1451 175 1289 1451 176 (n,gamma) cross section 1289 1451 177 the cross section was assumed to be 1/v below 100 ev with 1289 1451 178 a 2200 m/sec cross section of 9.5 mb. it was then extrapolated 1289 1451 179 linearly on a log-log basis to 0.1 mb at 1 kev, and then held 1289 1451 180 constant at this value up to 20 mev. 1289 1451 181 1289 1451 182 (n,x gamma) cross section 1289 1451 183 gamma rays in be-9 are produced by the (n,gamma) and the 1289 1451 184 (n,t) reactions. at thermal energies, ref. 2415 quotes gamma ray 1289 1451 185 energies of 0.8535, 2.59, 3.368, 3.444, 5.958 and 6.81 mev and 1289 1451 186 the corresponding (n,x gamma) cross sections. 1289 1451 187 the photon spectrum from this work was used at all neutron 1289 1451 188 energies. the multiplicity varied with neutron energy as 1289 1451 189 m(e)=m(0)(ecm+q)/q. m(0) is the multiplicity at thermal 1289 1451 190 and q is the (n,gamma) q value. this combination of spectra 1289 1451 191 and multiplicity conserves energy. there are no doubt other 1289 1451 192 levels in be-10 with energies greater than 6.81 mev excited as 1289 1451 193 the incident neutron energy is increased. the energies of the 1289 1451 194 higher states have not yet been determined so we use this 1289 1451 195 artifact to conserve energy. the component resulting from the 1289 1451 196 (n,t) reaction is equal to the (n,t1) cross section since its 1289 1451 197 multiplicity is unity. 1289 1451 198 1289 1451 199 references 1289 1451 200 (reference numbers quoted here refer to data in the lll 1289 1451 201 experimental neutron cross section library. see ucrl-50400, vol. 1289 1451 202 2 and 3 for comments and indexes to the data). 1289 1451 203 63. phys. rev. 80, 1011 (1950) c.k. bockelman. 1289 1451 204 72. phys. rev. 84, 69 (1951) c.k. bockelman, d.w. miller, 1289 1451 205 r.k. adair, h.h. barschall. r 1289 1451 206 86. phys. rev. 89, 80 (1953) m.e. battat, f.l. ribe. 1289 1451 207 92. private communication (1954) p.h. stelson. 1289 1451 208 107. phys. rev. 94, 651 (1954) c.f. cook, t.w. bonner. 1289 1451 209 121. phys. rev. 98, 669 (1955) j.d. seagrave, r.l. henkel. 1289 1451 210 151. phys. rev. 104, 1319 (1956) j.r. beyster, m. walt, 1289 1451 211 e.w. salmi. 1289 1451 212 160. phys. rev. 106, 1252 (1957) p.h. stelson, e.c. campbell. 1289 1451 213 231. anl-5567 (1956) a. langsdorf, jr., r.o. lane, j.e. monahan,1289 1451 214 see also, anl-5554 p. 22 (1956), phys. rev. 107, 1077 1289 1451 215 (1957), anl-5567 (rev.) (1961). 1289 1451 216 296. phys. rev. 98, 677 (1955) m. walt, j.r. beyster. 1289 1451 217 336. proc. phys. soc. (london) 64, 388 (1951) g.h. st afford. 1289 1451 218 356. phys. rev. 111, 1155 (1958) m.h. macgregor, w.p. ball, 1289 1451 219 r. booth. 1289 1451 220 402. phys. rev. 110, 1439 (1959) m.p. nakada, j.d. anderson, 1289 1451 221 c.c. gardner, c. wong. 1289 1451 222 494. doklady akad. nauk s.s.s.r. 119, 914 (1958) s.s. vasilev, 1289 1451 223 v.v. kumarov, a.m. popova, see also, j. exptl. theoret. 1289 1451 224 phys. (ussr) 33, 527 (1957). 1289 1451 225 496. phys. rev. 112, 1264 (1958) m.e. wyman, e.m. fryer, 1289 1451 226 m.m. thorpe. 1289 1451 227 500. phys. rev. 114, 1584 (1959) j.b. marion, j.s. levin, 1289 1451 228 l. cranberg. 1289 1451 229 571. anl-6172 (1960) r.o. lane, a.s. langsdorf, jr., 1289 1451 230 j.e. monahan, a.j. elwyn, see also, ann. phys. (n.y.) 12, 1289 1451 231 135 (1961). 1289 1451 232 605. ucrl-5596)(1959) j. benveniste, a.c. mitchell, 1289 1451 233 c.d. schrader, j.h. zenger, see also, nuclear phys. 19, 52 1289 1451 234 (1960). 1289 1451 235 650. j. exptl. theoret. phys. (ussr) 40, 1244 (1961) 1289 1451 236 s.a. myachkova, v.p. perelygin. 1289 1451 237 673. phys. rev. 120, 521 (1960) j.m. peterson, a. bratenahl, 1289 1451 238 j.p. stoering. 1289 1451 239 682. phys. rev. 123, 209 (1961) d.b. fossan, r.l. walter, 1289 1451 240 w.e. wilson, h.h. barschall. 1289 1451 241 720. private communication (1962) e.g. bilpuch, j.a. farrell, 1289 1451 242 g.c. kyker, jr., p.b. parks, h. newson. 1289 1451 243 733. nuclear ph ys. 23, 122 (1961) r. bass, t.w. bonner, 1289 1451 244 h.p.haenni. 1289 1451 245 750. private communication (1967) d.g. foster, jr., 1289 1451 246 d.w. glasgow, see also, hw-73116 (1962), hw-77311 (1963), 1289 1451 247 phys. rev. c, 3, 576 (1971), phys. rev. c, 3, 604 (1971). 1289 1451 248 763. nuclear phys. 129, 305 (1969) m. holmberg, j. hansen, see 1289 1451 249 also, iaea conference on nuclear data, paris, paper 1289 1451 250 cn-23/18 (1966). 1289 1451 251 772. compt. rend. 255, 277 (1962) a. perrin, g. surget, 1289 1451 252 c. thibault, f. verriere. 1289 1451 253 913. phys. rev. 132, 328 (1963) d.e. albuger. 1289 1451 254 945. ornl-2610 p. 14 (1958) h.o. cohn, j.l. fowler, see also, 1289 1451 255 bull. am. phys. soc. 3, 305 (1958). 1289 1451 256 1002. private communication (1954) c.t. hibdon, a. langsdorf. 1289 1451 257 1642. bull. am. phys. soc. 4, 385 (1959) j.l. fowler, h.o. cohn. 1289 1451 258 1643. doklady akad. nauk s.s.s.r. 158, 574 (1964) g.v. gorlov, 1289 1451 259 n.s. lebedeva, v.m. morozov, see also, yad. fiz. 5, 910 1289 1451 260 (1967). 1289 1451 261 1645. private communication (1960) j.s. levin, l. cranberg, see 1289 1451 262 also, wash-1028 p. 26 (1960), wash-1029 p. 44 (1960). 1289 1451 263 1646. private communication (1961) d.d. phillips. 1289 1451 264 1647. phys. rev. 133, 409 (1964) r.o. lane, a.j. elwyn, 1289 1451 265 a. langsdorf, jr. 1289 1451 266 2367. nuclear phys. 96, 476 (1967) g. paic, d. rendic, p. tomas. 1289 1451 267 2415. ga-10248 (dasa-2570) (1970) n.c. rasmussen, v.j. orphan, 1289 1451 268 t.l. harper, j. cunningham, s.a. ali. 1289 1451 269 2585. private communication (1966) r. bouchez, see also, iaea 1289 1451 270 conference on nuclear data, paris, paper cn-23/75 (1966). 1289 1451 271 2595. conference on neutron cross section technology, 1289 1451 272 washington d. c., vol. 1, p. 169 (1968) j.r.p. eaton, 1289 1451 273 j. walke . 1289 1451 274 3088. conference on neutron cross section technology, 1289 1451 275 washington d. c., p. 851 (1968) c.h. johnson, f.x. haas, 1289 1451 276 j.l. fowler, f.d. martin, r.l. kernell, h.o. cohn. 1289 1451 277 3101. z. naturforsch. 24, 289 (1969) w. scobel. 1289 1451 278 3106. np-17794 (1968) j. roturier, see also, compt. rend. 260, 1289 1451 279 4491 (1965), bnl-400, 3rd ed. (1970). 1289 1451 280 3320. atomkernenergie 20,309 (1972) m. bloser 1289 1451 281 3321. univ. of birmingham dept. of phys. rept. 73-02 (1973) 1289 1451 282 d.r. weaver, j. walker 1289 1451 283 1 451 324 1289 1451 284 2 151 4 1289 1451 285 3 1 84 1289 1451 286 3 2 21 1289 1451 287 3 6 8 1289 1451 288 3 7 10 1289 1451 289 3 8 7 1289 1451 290 3 9 5 1289 1451 291 3 46 8 1289 1451 292 3 47 10 1289 1451 293 3 48 7 1289 1451 294 3 49 5 1289 1451 295 3 102 56 1289 1451 296 3 103 5 1289 1451 297 3 104 6 1289 1451 298 3 105 6 1289 1451 299 3 107 8 1289 1451 300 3 251 10 1289 1451 301 3 252 10 1289 1451 302 3 253 10 1289 1451 303 3 740 5 1289 1451 304 3 741 6 1289 1451 305 4 2 176 1289 1451 306 4 6 10 1289 1451 307 4 7 100 1289 1451 308 4 8 10 1289 1451 309 4 9 10 1289 1451 310 4 46 218 1289 1451 311 4 47 146 1289 1451 312 4 48 57 1289 1451 313 4 49 49 1289 1451 314 5 46 383 1289 1451 315 5 47 396 1289 1451 316 5 48 251 1289 1451 317 5 49 202 1289 1451 318 12 102 4 1289 1451 319 12 741 4 1289 1451 320 14 102 1 1289 1451 321 14 741 1 1289 1451 322 15 102 22 1289 1451 323 15 741 12 1289 1451 324 1289 1 0 325 1289 0 0 326 4.00900+ 3 8.93480+ 0 0 0 1 01289 2151 327 4.00900+ 3 1.00000+ 0 0 0 1 01289 2151 328 1.00000- 4 2.00000+ 7 0 0 0 01289 2151 329 1.50000+ 0 6.90985- 1 0 0 0 01289 2151 330 1289 2 0 331 1289 0 0 332 4.00900+ 3 8.93480+ 0 0 0 0 01289 3 1 333 0.00000+ 0 0.00000+ 0 0 0 1 2411289 3 1 334 241 2 1289 3 1 335 1.00000- 5 6.47780+ 0 2.00000- 5 6.33780+ 0 3.00000- 5 6.27590+ 01289 3 1 336 4.00000- 5 6.23890+ 0 6.00000- 5 6.19510+ 0 8.00000- 5 6.16890+ 01289 3 1 337 1.00000- 4 6.15110+ 0 1.14220- 4 6.14140+ 0 1.29740- 4 6.13270+ 01289 3 1 338 1.47360- 4 6.12450+ 0 1.67380- 4 6.11680+ 0 1.89080- 4 6.10990+ 01289 3 1 339 2.12400- 4 6.10370+ 0 2.38600- 4 6.09780+ 0 2.68030- 4 6.09230+ 01289 3 1 340 2.99430- 4 6.08730+ 0 3.34510- 4 6.08260+ 0 3.73690- 4 6.07820+ 01289 3 1 341 4.15160- 4 6.07420+ 0 4.61240- 4 6.07040+ 0 5.12420- 4 6.06680+ 01289 3 1 342 5.66150- 4 6.06350+ 0 6.25500- 4 6.06040+ 0 6.91080- 4 6.05750+ 01289 3 1 343 7.63530- 4 6.05470+ 0 8.43580- 4 6.05200+ 0 9.26880- 4 6.04960+ 01289 3 1 344 1.01840- 3 6.04730+ 0 1.11890- 3 6.04520+ 0 1.22260- 3 6.04320+ 01289 3 1 345 1.33590- 3 6.04130+ 0 1.45970- 3 6.03950+ 0 1.59500- 3 6.03780+ 01289 3 1 346 1.74280- 3 6.03620+ 0 1.89380- 3 6.03470+ 0 2.05790- 3 6.03330+ 01289 3 1 347 2.23610- 3 6.03200+ 0 2.42990- 3 6.03070+ 0 2.62580- 3 6.02950+ 01289 3 1 348 2.85330- 3 6.02830+ 0 3.10050- 3 6.02710+ 0 3.36910- 3 6.02600+ 01289 3 1 349 3.66090- 3 6.02500+ 0 3.97810- 3 6.02400+ 0 4.29880- 3 6.02300+ 01289 3 1 350 4.64550- 3 6.02220+ 0 5.02000- 3 6.02130+ 0 5.42480- 3 6.02050+ 01289 3 1 351 5.82980- 3 6.01980+ 0 6.29990- 3 6.01900+ 0 6.77030- 3 6.01840+ 01289 3 1 352 7.81900- 3 6.01710+ 0 9.03010- 3 6.01590+ 0 1.03710- 2 6.01480+ 01289 3 1 353 1.19120- 2 6.01380+ 0 1.36050- 2 6.01300+ 0 1.54540- 2 6.01220+ 01289 3 1 354 1.75530- 2 6.01140+ 0 1.98280- 2 6.01070+ 0 2.23970- 2 6.01010+ 01289 3 1 355 2.53000- 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